Layered Composites for High Tan Delta Plateau over Wide Temperature Range.

Tan Delta reflects the viscoelastic behavior of materials, particularly polymers. In most cases, a high Tan Delta value is associated with transitions (such as glass transition or melting), enabling effective damping properties near these temperature ranges. However, achieving a high Tan Delta over a broad temperature range is challenging, particularly for engineering applications that involve significant temperature fluctuations. This paper presents a straightforward method using layered composites, where a polymer layer is sandwiched between two highly stretchable elastic fabrics, to achieve a wide Tan Delta plateau (TDP) across a broad temperature range. The three-layer configuration consists of a polymer core embedded between two elastic layers. All samples prepared with this architecture consistently exhibit the TDP. Further investigations examine the influence of factors such as the number of layers and the stretchability of the elastic fabrics. The results demonstrate that the TDP can be effectively tailored for engineering applications using this layered design.