ArticleNature communications2025
Entropy engineering activation of UiO-66 for boosting catalytic transfer hydrogenation.
Article in Nature communications, 2025. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 4 papers.
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Who cites it
4 citing papers in PubMed.
- Caging Lithium Deposition: High-Entropy Metal-Organic Framework Interfaces for Anode-Free Batteries.Advanced materials (Deerfield Beach, Fla.) · 2026Article
- Entropy-Engineered Multi-Metallic MOFs Unlock High-Performance Ammonium-Ion Storage.Small (Weinheim an der Bergstrasse, Germany) · 2026Article
- [H]-mediated enhancement of the Fenton reaction over a Pd/UiO-66(Zr)-FTurkish journal of chemistry · 2026Article
- Triple Redox-Enabled High-Entropy Metal-Organic Coordination Driving High-Performance Aqueous Zinc-Ion Batteries.Advanced science (Weinheim, Baden-Wurttemberg, Germany) · 2025Article
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Authors and funding
5 authors.
Funding
Abstract
High-entropy metal-organic frameworks (HE-MOFs) hold promise as versatile materials, yet current rare examples are confined to low-valence elements in the fourth period, constraining their design and optimization for diverse applications. Here, a novel high-entropy, defect-rich and small-sized (32 nm) UiO-66 (ZrHfCeSnTi HE-UiO-66) has been synthesized for the first time, leveraging increased configurational entropy to achieve high tolerance to doping with diverse metal ions. The lattice distortion of HE-UiO-66 induces high exposure of metal nodes to create coordination unsaturated metal sites with a concentration of 322.4 μmol/g, which increases the abundance of Lewis acid-base sites, thereby achieving a significant improvement in the performance of the catalytic transfer hydrogenation (CTH) reaction. Systematic investigation manifests that the special electronic structure of HE-UiO-66 enhances the interaction and bonding with substrate molecules and reduces the energy barrier of the hydrogen transfer process. Our approach offers a new strategy for constructing coordination unsaturated metal sites in MOFs.
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Registered trials
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