ArticleLangmuir : the ACS journal of surfaces and colloids2025
Deformation, Rupture, and Morphology Hysteresis of Copolymer Nanovesicles in Uniform Shear Flow.
Article in Langmuir : the ACS journal of surfaces and colloids, 2025. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Not yet cited in PubMed.
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Abstract
Copolymer nanovesicles are used extensively in chemical processes and biomedical applications in which they are subjected to dynamic flow environments. Flow-induced vesicle deformation, fragmentation, and reorganization modify the energetic (e.g., polymer-solvent interfacial area) and entropic (e.g., copolymer chain configuration) contributions to the solution free energy. Equilibration of a deformed morphology by flow cessation could reorganize the system into a self-assembled state, which is different from the parent structure through a local free energy minimization pathway. We perform nonequilibrium molecular dynamics simulations to investigate morphology evolution in uniform shear flow of a unilamellar nanovesicle formed by the self-assembly of amphiphilic triblock copolymers in an aqueous solution. Flow strength is characterized by the Weissenberg number
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