ArticleProceedings of the National Academy of Sciences of the United States of America2025
Fast-chargeable lithium-ion batteries by μ-Si anode-tailored full-cell design.
Article in Proceedings of the National Academy of Sciences of the United States of America, 2025. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 6 papers.
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Who cites it
6 citing papers in PubMed.
- Toward interface-adaptive silicon anodes: From 3D SEI to dynamic coupled interphases.Innovation (Cambridge (Mass.)) · 2026Review
- Mechanically Adaptive Polyrotaxane Interlayers for Low-Pressure High Energy Density Sulfide-Based All-Solid-State Batteries.Angewandte Chemie (International ed. in English) · 2026Article
- Study of Dangling Bond States in Magnetron-Sputtered a-Si Thin Films via Parametrization Using a Single UV-Vis-NIR Transmittance Spectrum.Molecules (Basel, Switzerland) · 2026Article
- Dynamic Evolution and Degradation of Silicon-Electrolyte Interfaces under Cycling via Chemical Potential-Controlled Molecular Dynamics.ACS applied materials & interfaces · 2026Article
- Maxwell Protocol for Non-Destructive Health Diagnosis of All-Solid-State Batteries.Angewandte Chemie (International ed. in English) · 2025Article
- High-performance anode-less all-solid-state batteries enabled by multisite nucleation and an elastic network.EES batteries · 2025Article
Corrections and comments
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Authors and funding
8 authors.
Funding
Abstract
Silicon (Si) anodes have long been recognized to significantly improve the energy density and fast-charging capability of lithium-ion batteries (LIBs). However, the implementation of these anodes in commercial LIB cells has progressed incrementally due to the immense volume change of Si across its full state-of-charge (SOC) range. Here, we report an anode-tailored full-cell design (ATFD), which incorporates micrometer-sized silicon (μ-Si) alone, for operation over a limited, prespecified SOC range identified as 30-70%. This range allows homogeneous (de)lithiation throughout the electrode, accompanied by an acceptable level of volume change. The ATFD-based cell exhibits 21.3% higher gravimetric energy density than that of its graphite-based counterpart in a commercial 18650 cylindrical cell and 84.6% capacity retention after 500 cycles even at a fast-charging rate of 3 C. This study indicates that the partial, intermediate SOC operation of the μ-Si anode can markedly increase the energy density and boost the fast-charging capability of a LIB cell, a challenging task in traditional cell engineering.
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