ArticleThe journal of physical chemistry. C, Nanomaterials and interfaces2024
Electrified Nanogaps under an AC Field: A Molecular Dynamics Study.
Article in The journal of physical chemistry. C, Nanomaterials and interfaces, 2024. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Not yet cited in PubMed.
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Abstract
The organization and dynamics of ions and water molecules at electrified solid-liquid interfaces are generally well understood under static fields, especially for macroscopic electrochemical systems. In contrast, studies involving alternating (AC) fields tend to be more challenging. In nanoscale systems, added complexity can arise from interfacial interactions and the need to consider ions and molecules explicitly. Here we use molecular dynamics (MD) simulations to investigate the behavior of NaCl aqueous solutions at different concentrations confined in nanogaps under AC fields ranging from 10 MHz to 10 GHz. We explore the impact of the gap size (2-60 nm) and of the solid material composing the electrode (silica, charged silica, or gold). Analysis of the transient and stable responses of the system shows that the total transverse dipole
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