ArticleNanophotonics (Berlin, Germany)2024
Linear optical properties of organic microcavity polaritons with non-Markovian quantum state diffusion.
Article in Nanophotonics (Berlin, Germany), 2024. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 4 papers.
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4 citing papers in PubMed.
- A fully solution-processed organic microcavity laser in the strong light-matter coupling regime.Nature communications · 2026Article
- Impact of light-matter coupling strength on the efficiency of microcavity OLEDs: a unified quantum master equation approach.Materials horizons · 2026Article
- Enhanced Delayed Fluorescence in Nonlocal Metasurfaces: The Role of Electronic Strong Coupling.ACS photonics · 2025Article
- Strong Coupling of Organic Molecules 2023 (SCOM23).Nanophotonics (Berlin, Germany) · 2024Article
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5 authors.
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Abstract
Hybridisation of the cavity modes and the excitons to polariton states together with the coupling to the vibrational modes determine the linear optical properties of organic semiconductors in microcavities. In this article we compute the refractive index for such system using the Holstein-Tavis-Cummings model and determine then the linear optical properties using the transfer matrix method. We first extract the parameters for the exciton in our model from fitting to experimentally measured absorption of a 2,7-bis[9,9-di(4-methylphenyl)-fluoren-2-yl]-9,9-di(4-methylphenyl) fluorene (TDAF) molecular thin film. Then we compute the reflectivity of such a thin film in a metal clad microcavity system by including the dispersive microcavity mode to the model. We compute susceptibility of the model systems evolving just a single state vector by using the non-Markovian quantum state diffusion. The computed location and height of the lower and upper polaritons agree with the experiment within the estimated errorbars for small angles
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