ArticleNanophotonics (Berlin, Germany)2024
Extracting accurate light-matter couplings from disordered polaritons.
Article in Nanophotonics (Berlin, Germany), 2024. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 9 papers.
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Who cites it
9 citing papers in PubMed.
- A macroscopic condensation theory for vibrational strong coupling effects.Nature communications · 2026Article
- Ab Initio Polariton Spectra of ZnTPP Molecules Collectively Coupled Inside an Optical Cavity.Journal of the American Chemical Society · 2026Article
- Interference-Induced Cavity Resonances and Imaginary Rabi Splitting.Nanophotonics (Berlin, Germany) · 2026Article
- Long-lived polaritonic coherence and polaron decoupling effects in 2D electronic spectra.Proceedings of the National Academy of Sciences of the United States of America · 2026Article
- Real-space observation of flat-band ultrastrong coupling between optical phonons and surface plasmon polaritons.Nature materials · 2026Article
- Polaritonic quantum matter.Nanophotonics (Berlin, Germany) · 2025Review
- Quantitative Modeling of Polaritonic Emission Using the Source Term Method.The journal of physical chemistry letters · 2025Article
- Room-temperature cavity exciton-polariton condensation in perovskite quantum dots.Nature communications · 2025Article
- Strong Coupling of Organic Molecules 2023 (SCOM23).Nanophotonics (Berlin, Germany) · 2024Article
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3 authors.
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Abstract
The vacuum Rabi splitting (VRS) in molecular polaritons stands as a fundamental measure of collective light-matter coupling. Despite its significance, the impact of molecular disorder on VRS is not fully understood yet. This study delves into the complexities of VRS amidst various distributions and degrees of disorder. Our analysis provides precise analytical expressions for linear absorption, transmission, and reflection spectra, along with a "sum" rule, offering a straightforward protocol for extracting accurate collective light-matter coupling values from experimental data. Importantly, our study cautions against directly translating large VRS to the onset of ultrastrong coupling regime. Furthermore, for rectangular disorder, we witness the emergence of narrow side bands alongside a broad central peak, indicating an extended coherence lifetime even in the presence of substantial disorder. These findings not only enhance our understanding of VRS in disordered molecular systems but also open avenues for achieving prolonged coherence lifetimes between the cavity and molecules via the interplay of collective coupling and disorder.
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