ArticleNanophotonics (Berlin, Germany)2024
A mixed perturbative-nonperturbative treatment for strong light-matter interactions.
Article in Nanophotonics (Berlin, Germany), 2024. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 6 papers.
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6 citing papers in PubMed.
- Quantized Plasmon Modes for Metallic Nanoparticles of Arbitrary Shape with a Generic Dielectric Function.The journal of physical chemistry letters · 2026Article
- Interference-Induced Cavity Resonances and Imaginary Rabi Splitting.Nanophotonics (Berlin, Germany) · 2026Article
- Incorporating QM/MM Molecular Dynamics Into the Few-Mode Quantization Approach for Light-Matter Interactions in Nanophotonic Structures.Nanophotonics (Berlin, Germany) · 2026Article
- Molecular Polarizability under Vibrational Strong Coupling.Journal of chemical theory and computation · 2025Article
- Radiative pumping vs vibrational relaxation of molecular polaritons: a bosonic mapping approach.Nature communications · 2025Article
- Strong Coupling of Organic Molecules 2023 (SCOM23).Nanophotonics (Berlin, Germany) · 2024Article
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Abstract
The full information about the interaction between a quantum emitter and an arbitrary electromagnetic environment is encoded in the so-called spectral density. We present an approach for describing such interaction in any coupling regime, providing a Lindblad-like master equation for the emitter dynamics when coupled to a general nanophotonic structure. Our framework is based on the splitting of the spectral density into two terms. On the one hand, a spectral density responsible for the non-Markovian and strong-coupling-based dynamics of the quantum emitter. On the other hand, a residual spectral density including the remaining weak-coupling terms. The former is treated nonperturbatively with a collection of lossy interacting discrete modes whose parameters are determined by a fit to the original spectral density in a frequency region encompassing the quantum emitter transition frequencies. The latter is treated perturbatively under a Markovian approximation. We illustrate the power and validity of our approach through numerical simulations in three different setups, thus offering a variety of scenarios for a full test, including the ultra-strong coupling regime.
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