Evidence map›Paper›PMID 39661727›Full record

ArticleAdvanced science (Weinheim, Baden-Wurttemberg, Germany)2025

Engineering p-Orbital States via Molecular Modules in All-Organic Electrocatalysts toward Direct Water Oxidation.

Li-Hong Yu, Xue-Feng Zhang, Zi-Ming Ye, Hong-Gang Du, Li-Dong Wang, Ping-Ping Xu, Yuhai Dou, Li-Ming Cao, Chun-Ting He

Abstract read
PubMed Full text at PMC Publisher
In one paragraph

Article in Advanced science (Weinheim, Baden-Wurttemberg, Germany), 2025. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 1 paper.

0numbers the graph read from it
0cells of the map it votes in
1citing papers in PubMed
–field-weighted citation impact
1 · What the graph read from it

What it found

Each row is one number read from the abstract, on the scale the paper reported it, with its interval. Left of the dashed line favours the treatment, right favours the comparator. Under each row is the sentence it came from. New to these charts? A ten-minute tutorial.

The abstract states no effect estimate the extractor could read, or names no intervention and outcome on the map, so this paper lights no cell and moves no belief. It is still indexed, cited and linked below.

2 · The registry

The trial behind it

Trials whose registry record cites this paper, or whose number appears in the abstract. A trial that started after this paper was published is citing it as background, not reporting it.

Neither the registry nor the abstract names a trial number. If this is a trial report, that itself is worth knowing.

3 · Its place in the literature

Who cites it

1 citing paper in PubMed.

  1. Article
4 · The record

Corrections and comments

PubMed lists nothing against this paper. Absence here is not a guarantee, only a check that was made.

5 · Who and what money

Authors and funding

9 authors.

Li-Hong YuKey Lab of Fluorine and Silicon for Energy Materials and Chemistry of Ministry of Education, College of Chemistry and Materials, Jiangxi Normal University, Nanchang, 330022, China.
Xue-Feng ZhangKey Lab of Fluorine and Silicon for Energy Materials and Chemistry of Ministry of Education, College of Chemistry and Materials, Jiangxi Normal University, Nanchang, 330022, China.
Zi-Ming YeDepartment of Chemistry, Northwestern University, Evanston, IL, 60208, USA.
Hong-Gang DuKey Lab of Fluorine and Silicon for Energy Materials and Chemistry of Ministry of Education, College of Chemistry and Materials, Jiangxi Normal University, Nanchang, 330022, China.
Li-Dong WangKey Lab of Fluorine and Silicon for Energy Materials and Chemistry of Ministry of Education, College of Chemistry and Materials, Jiangxi Normal University, Nanchang, 330022, China.
Ping-Ping XuKey Lab of Fluorine and Silicon for Energy Materials and Chemistry of Ministry of Education, College of Chemistry and Materials, Jiangxi Normal University, Nanchang, 330022, China.
Yuhai DouInstitute of Energy Materials Science, University of Shanghai for Science and Technology, Shanghai, 200093, China.
Li-Ming CaoKey Lab of Fluorine and Silicon for Energy Materials and Chemistry of Ministry of Education, College of Chemistry and Materials, Jiangxi Normal University, Nanchang, 330022, China.
Chun-Ting HeKey Lab of Fluorine and Silicon for Energy Materials and Chemistry of Ministry of Education, College of Chemistry and Materials, Jiangxi Normal University, Nanchang, 330022, China.ORCID https://orcid.org/0000-0003-0009-7693

Funding

Jiangxi Provincial Natural Science Foundation 20224ACB214001Jiangxi Provincial Natural Science Foundation 20232ACB213009Jiangxi Provincial Natural Science Foundation 20242BAB26033Jiangxi Provincial Natural Science Foundation 20242BAB26046Jiangxi Provincial Natural Science Foundation 20243BCE51069National Natural Science Foundation of China 22161021National Natural Science Foundation of China 22265012National Natural Science Foundation of China 22375079National Natural Science Foundation of China 22379057
6 · The paper itself

Abstract

Oxygen evolution reaction (OER) is an indispensable anode reaction for sustainable hydrogen production from water electrolysis, yet overreliance on metal-based catalysts featured with vibrant d-electrons. It still has notable gap between metal-free and metal-based electrocatalysts, due to lacking accurate and efficient p-band regulation methods on non-metal atoms. Herein, a molecular modularization strategy is proposed for fine-tuning the p-orbital states of series metal-free covalent organic frameworks (COFs) for realizing OER performance beyond benchmark precious metal catalysts. Optimized combination of benzodioxazole/benzodiimide-based building blocks achieves an impressive applied potential of 1.670 ± 0.004 V versus reversible hydrogen electrode (RHE) and 1.735 ± 0.006 V versus RHE to deliver enhanced current densities of 0.5 and 1.0 A cm

Indexed as

catalytic mechanismcovalent organic frameworks (COFs)electrocatalystsoxygen evolution reaction (OER)

Identifiers

PMID39661727
PMCPMC11792050

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Read under generation 80e0d062 · epoch 390. Bibliography from PubMed, PubMed Central and OpenAlex; grants from NIH RePORTER; trial links from ClinicalTrials.gov; estimates, votes and beliefs from the OpenQuestion graph.