ArticleScience advances2024
Turing covalent organic framework membranes via heterogeneous nucleation synthesis for organic solvent nanofiltration.
Article in Science advances, 2024. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 13 papers.
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Who cites it
13 citing papers in PubMed.
- Hydration channel engineering in Tröger's base-POP membranes for mono/multivalent cation and anion discrimination.Science advances · 2026Article
- Precise molecular sieving in polycrystalline covalent organic framework membranes.Science advances · 2026Article
- Heteroatom-Mediated Covalent Organic Framework Membranes With Nitrogen-Enriched Nanochannels for Efficient Desalination.Advanced science (Weinheim, Baden-Wurttemberg, Germany) · 2026Article
- Pre-Crosslinked Network-Mediated Dual Exchange Enables Boosting Chiroptical Activity and Decoupled Two-Level Chirality in Covalent Organic Frameworks.Angewandte Chemie (International ed. in English) · 2026Article
- Reversible Exfoliation-Aggregation Dynamics in Ionic COFs for Tunable Interfacial Catalysis.Advanced science (Weinheim, Baden-Wurttemberg, Germany) · 2026Article
- Covalent Organic Framework Membranes through Sequential Imine Exchange for Precise Molecular Separation.Nano-micro letters · 2026Article
- Stable porous graphene oxide membranes enabled by confined growth of 2D MOF nanosheets for high-performance desalination.Science advances · 2026Article
- Turing-patterned TaNature communications · 2026Article
- Microenvironment-Engineered Biocatalytic Metal-Organic Framework Nanomotors for Selective and Transformative Water Decontamination.Nano-micro letters · 2026Article
- Flexible High-Aspect-Ratio COF Nanofibers: Defect-Engineered Synthesis, Superelastic Aerogels, and Uranium Extraction Applications.Nano-micro letters · 2026Article
- Article
- Asymmetric ionic covalent organic framework membranes with tunable Turing patterns prepared via ion regulated strategy.Nature communications · 2025Article
- Light-activated 3D covalent organic framework membranes with adaptive pores for COScience advances · 2025Article
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Authors and funding
8 authors.
Funding
No grant is acknowledged in the PubMed record.
Abstract
Although covalent organic frameworks (COFs) demonstrate notable potential for developing advanced separation membranes, contemporary COF membranes still lack controlled stacking and highly efficient sieving. Here, Turing-architecture COF membranes were constructed by engineering a reaction-diffusion assembly process via heterogeneous nucleation synthesis with tannic acid (TA). TA covalently binds with amine monomers to form a composite precursor with increased reactivity and decreased diffusivity. This altered the pathway of Schiff base reactions with aldehyde monomers, fulfilling suitable reaction-diffusion conditions, and ultimately formed the labyrinthine stripe or spot-patterned Turing COF film with controlled stacking and uniform pore structure. This endows our COF membrane with highly efficient molecule sieving ability for organic solvent nanofiltration while exhibiting a flux that is 621% greater than that of commercial membranes. Thus, this study provides a paradigm for the in situ synthesis of highly efficient COF membranes for diversely sustainable separations.
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Registered trials
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