ArticleAdvanced materials (Deerfield Beach, Fla.)2025
Hydride-Induced Reconstruction of Pd Electrode Surfaces: A Combined Computational and Experimental Study.
Article in Advanced materials (Deerfield Beach, Fla.), 2025. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 8 papers.
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Who cites it
8 citing papers in PubMed.
- Hydride-induced palladium self-diffusion and surface restructuring on Pd(111).Nature communications · 2026Article
- The Applications of Machine Learning in Micro-Nano Materials Research: From High-Throughput Screening to Intelligent Design.Small (Weinheim an der Bergstrasse, Germany) · 2026Review
- Subsurface hydrogen as a hidden driver of copper surface reconstruction in CONational science review · 2026Article
- Local Activity and Selectivity Hotspots in Cu-Pt Model Thin-Film Electrocatalysts for Oxygen Reduction.Small methods · 2026Article
- Revealing Catalytic Properties of Palladium/Gold Systems toward Hydrogen Evolution, Oxidation, and Absorption with Scanning Electrochemical Microscopy.ACS catalysis · 2025Article
- Palladium Nanocubes with {100} Facets for Hydrogen Evolution Reaction: Synthesis, Experiment and Theory.Small (Weinheim an der Bergstrasse, Germany) · 2025Article
- Development of an atomic cluster expansion potential for iron and its oxides.npj computational materials · 2025Article
- Hydride-Induced Reconstruction of Pd Electrode Surfaces: A Combined Computational and Experimental Study.Advanced materials (Deerfield Beach, Fla.) · 2025Article
Corrections and comments
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Authors and funding
18 authors.
Funding
Abstract
Designing electrocatalysts with optimal activity and selectivity relies on a thorough understanding of the surface structure under reaction conditions. In this study, experimental and computational approaches are combined to elucidate reconstruction processes on low-index Pd surfaces during H-insertion following proton electroreduction. While electrochemical scanning tunneling microscopy clearly reveals pronounced surface roughening and morphological changes on Pd(111), Pd(110), and Pd(100) surfaces during cyclic voltammetry, a complementary analysis using inductively coupled plasma mass spectrometry excludes Pd dissolution as the primary cause of the observed restructuring. Large-scale molecular dynamics simulations further show that these surface alterations are related to the creation and propagation of structural defects as well as phase transformations that take place during hydride formation.
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Registered trials
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