ArticleJournal of the American Chemical Society2024
Single-Crystal Dynamic Covalent Organic Frameworks for Adaptive Guest Alignments.
Article in Journal of the American Chemical Society, 2024. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 9 papers.
What it found
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Who cites it
9 citing papers in PubMed.
- Cooperative stabilization mechanism and electrostatic evolution in the zero dimensional arsenolite cluster aggregates: a first principles investigation.RSC advances · 2026Article
- Solvent-Induced Structural Modulation in Nanoscale Covalent Organic Frameworks Enables High-Performance NOAngewandte Chemie (International ed. in English) · 2026Article
- Structure-Dynamics-Property Relationship Reveals the Origin of Porous Integrity in Imine-Linked Covalent Organic Frameworks.Journal of the American Chemical Society · 2026Article
- Thermoresponsive and xenon-triggered gate-opening in flexible three-dimensional covalent organic framework for selective xenon capture.Nature communications · 2026Article
- Single Crystals of Perylene Diimide-Based Two-Dimensional Covalent Organic Frameworks.Advanced materials (Deerfield Beach, Fla.) · 2026Article
- Large Multichannel Architectures in Three-Dimensional Covalent Organic Frameworks for Efficient Guest Diffusion.Journal of the American Chemical Society · 2026Article
- Dynamic covalent organic frameworks.Chemical science · 2026Review
- Radial growth of twist-stacked covalent organic framework nanofibers.Nature communications · 2025Article
- Synthesis and crystal structure ofActa crystallographica. Section E, Crystallographic communications · 2025Article
Corrections and comments
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Authors and funding
9 authors.
Funding
No grant is acknowledged in the PubMed record.
Abstract
Dynamic 3D covalent organic frameworks (COFs) have shown a concerted structural transformation upon adaptive guest inclusion. However, the origin of the conformational mobility and the host-guest adaptivity remain conjecture of the pedal motions of revolving imine linkages, often without considering the steric hindrance from the interwoven frameworks. Here, we present atomic-level observation of the rotational and translational dynamics in single-crystal COF-300 upon adaptive guest inclusion of various organic molecules, featuring multiple rotamers of covalent linkages and switchable interframework noncovalent interactions. Specifically, we developed a diffusion gradient transimination protocol to facilitate the growth of COF single crystals, enabling a high-resolution X-ray diffraction structural analysis. We uncovered metastable and low-symmetry intermediate phases from contracted to expanded phases during structural evolution. We identified torsion angles in the terephthalaldehyde diimine motifs that switch from
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Registered trials
Read under generation 80e0d062 · epoch 390. Bibliography from PubMed, PubMed Central and OpenAlex; grants from NIH RePORTER; trial links from ClinicalTrials.gov; estimates, votes and beliefs from the OpenQuestion graph.