ArticleCommunications chemistry2024
Rotaxane-catalyzed aerobic oxidation of primary alcohols.
Article in Communications chemistry, 2024. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 2 papers.
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Who cites it
2 citing papers in PubMed.
- Design strategies and emerging applications for mechanically interlocked molecules.Communications chemistry · 2025Article
- Influence of Protonation and Iron(II) Complexation on Magnetic Interactions in Spin-Labeled Mechanically Interlocked Molecules.Chemistry (Weinheim an der Bergstrasse, Germany) · 2025Article
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Authors and funding
11 authors.
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Abstract
Nitroxide radicals are widely utilized as catalysts for the oxidation of primary alcohols. Here, the aerobic catalytic oxidation cycle of nitroxide radicals has been implemented within a mechanically interlocked rotaxane architecture consisting of a paramagnetic crown ether, which is confined by a molecular axle containing a dialkylammonium station and a 1,2,3-triazole unit. The rotaxane is engineered to exploit the oxidation of a primary alcohol: the primary catalyst is the wheel, a nitroxide radical capable of altering its oxidation state during the catalytic cycle, while the co-oxidant is the Cerium(IV)/O
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