ArticleAccounts of chemical research2024
n-Type Conjugated Polymers Based on Double B←N Bridged Bipyridine Unit.
Article in Accounts of chemical research, 2024. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Not yet cited in PubMed.
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Abstract
ConspectusBoth p-type conjugated polymers and n-type conjugated polymers are required for organic optoelectronic devices, such as organic solar cells (OSCs), organic field-effect transistors (OFETs), organic thermoelectrics (OTEs), etc. The development of n-type conjugated polymers lags far behind that of the p-type counterparts in view of material diversity and optoelectronic device performance. This is mainly due to the lack of strong electron-withdrawing building blocks, which are always based on the imide unit. Double boron-nitrogen coordination bond (B←N) bridged bipyridine (BNBP), which was first developed in 2016, is an alternative kind of electron-withdrawing building block based on a B←N unit. BNBP itself possesses a planar and fixed configuration, low-lying electronic energy levels, strong fluorescence, and facile functionalization. A family of BNBP-based conjugated polymers has been developed. They show excellent and tunable optoelectronic properties, such as high electron mobility, low-lying and tunable lowest unoccupied molecular orbital (LUMO) energy level (
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