ArticleThe journal of physical chemistry. C, Nanomaterials and interfaces2024
Band Diagram Insights into the Kinetic and Thermodynamic Engineering of Tandem Photocatalytic Cells.
Article in The journal of physical chemistry. C, Nanomaterials and interfaces, 2024. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Not yet cited in PubMed.
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Abstract
In this work, we theoretically investigate the impact of kinetic and thermodynamic properties on the performance of photocatalytic cells operating in an unassisted tandem configuration, including electron affinity and ionization energies, recombination rates, and reaction rates. To this end, we present general rules and metrics for identifying and isolating the origin of an observed shift in the onset potential at either the photoanode or the photocathode of these devices. The correlation between kinetic and thermodynamic shifts in the onset potential is demonstrated through the use of band diagrams and key comparable features within readily accessible characterization tools: current-voltage plots are taken both under illumination and in the dark and further coupled with Mott-Schottky plots. To illustrate this conceptual framework, a model system comprised of a p-type doped BiVO
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