ArticleNature photonics2024
Chiral topological light for detection of robust enantiosensitive observables.
Article in Nature photonics, 2024. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 7 papers.
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Who cites it
7 citing papers in PubMed.
- Pulse-Duration-Sensitive High Harmonics and Attosecond Locally Chiral Near Fields from a Chiral Topological Weyl Semimetal.Nano letters · 2026Article
- Probing Broken Time-Reversal Symmetry in 2D Materials with Tailored-Light Photocurrent Generation.ACS nano · 2026Article
- Quantum-elevated chiral discrimination for biomolecules.Science advances · 2026Article
- Symmetries and selection rules in photoelectron chiral dichroism.Proceedings of the National Academy of Sciences of the United States of America · 2025Article
- Unidirectional perfect absorption induced by chiral coupling in spin-momentum locked waveguide magnonics.Nature communications · 2025Article
- Rotatum of light.Science advances · 2025Article
- Chiral topological light for detection of robust enantiosensitive observables.Nature photonics · 2024Article
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Authors and funding
7 authors.
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Abstract
The topological response of matter to electromagnetic fields is a highly demanded property in materials design and metrology due to its robustness against noise and decoherence, stimulating recent advances in ultrafast photonics. Embedding topological properties into the enantiosensitive optical response of chiral molecules could therefore enhance the efficiency and robustness of chiral optical discrimination. Here we achieve such a topological embedding by introducing the concept of chiral topological light-a light beam which displays chirality locally, with an azimuthal distribution of its handedness described globally by a topological charge. The topological charge is mapped onto the azimuthal intensity modulation of the non-linear optical response, where enantiosensitivity is encoded into its spatial rotation. The spatial rotation is robust against intensity fluctuations and imperfect local polarization states of the driving field. Our theoretical results show that chiral topological light enables detection of percentage-level enantiomeric excesses in randomly oriented mixtures of chiral molecules, opening a way to new, extremely sensitive and robust chiro-optical spectroscopies with attosecond time resolution.
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