ArticleAdvanced science (Weinheim, Baden-Wurttemberg, Germany)2025
Surface Planarization-Epitaxial Growth Enables Uniform 2D/3D Heterojunctions for Efficient and Stable Perovskite Solar Modules.
Article in Advanced science (Weinheim, Baden-Wurttemberg, Germany), 2025. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 7 papers.
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Who cites it
7 citing papers in PubMed.
- Thermally Independent Interfacial Reconstruction for Phase-Pure n = 1 2D Perovskites With Mixed-Orientation Surface Architecture.Advanced materials (Deerfield Beach, Fla.) · 2026Article
- Precise Management of n-Value Distribution at the 2D/3D Interface Enabling Efficient Wide-Bandgap Perovskite Solar Cells.Advanced science (Weinheim, Baden-Wurttemberg, Germany) · 2026Article
- Perovskite Heterostructures for Optoelectronic Applications.Advanced materials (Deerfield Beach, Fla.) · 2026Review
- Synergistic energy and charge transfer dynamics in LD/3D perovskite heterojunctions for optoelectronic applications.Chemical science · 2026Review
- Recent progress in enhancing built-in electric fields of perovskite solar cells via junction engineering.Beilstein journal of nanotechnology · 2026Review
- In Situ Epitaxial Quantum Dot Passivation Enables Highly Efficient and Stable Perovskite Solar Cells.Nanomaterials (Basel, Switzerland) · 2025Article
- Surface Planarization-Epitaxial Growth Enables Uniform 2D/3D Heterojunctions for Efficient and Stable Perovskite Solar Modules.Advanced science (Weinheim, Baden-Wurttemberg, Germany) · 2025Article
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14 authors.
Funding
Abstract
Two-dimensional/three-dimensional (2D/3D) halide perovskite heterojunctions are widely used to improve the efficiency and stability of perovskite solar cells. However, interfacial defects between the 2D and 3D perovskites and the poor coverage of the 2D capping layer still hinder long-term stability and homogeneous charge extraction. Herein, a surface planarization strategy on 3D perovskite is developed that enables an epitaxial growth of uniform 2D/3D perovskite heterojunction via a vapor-assisted process. The homogeneous charge extraction and suppression of interfacial nonradiative recombination is achieved by forming a uniform 2D/3D interface. As a result, a stabilized power output efficiency of 25.97% is achieved by using a 3D perovskite composition with a bandgap of 1.55 eV. To demonstrate the universality of the strategy applied for different perovskites, the champion device based on a 1.57 eV bandgap 3D perovskite results in an efficiency of 25.31% with a record fill factor of 87.6%. Additionally, perovskite solar modules achieve a designated area (24.04 cm
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