ArticleAdvanced science (Weinheim, Baden-Wurttemberg, Germany)2024
High-Density Atomic Level Defect Engineering of 2D Fe-Based Metal-Organic Frameworks Boosts Oxygen and Hydrogen Evolution Reactions.
Article in Advanced science (Weinheim, Baden-Wurttemberg, Germany), 2024. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 8 papers.
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Who cites it
8 citing papers in PubMed.
- Interface Engineering in MOF-Derived NiOOH/FeOOH Heterostructures: Boosting OER Performance via Lattice Oxygen Redox Regulation and AEM/LOM Synergy.Small (Weinheim an der Bergstrasse, Germany) · 2026Article
- Interfacial Covalent Bonds Between Fe-MoSSmall (Weinheim an der Bergstrasse, Germany) · 2026Article
- Ligand-Intercalated MOFs Enable Reaction-Pathway Engineering in Biomass Electrooxidation via Steric and π-Electronic Microenvironment Control.Angewandte Chemie (International ed. in English) · 2026Article
- Fe metal-organic framework-derived heterojunction for metabolic diagnosis of thymic epithelial tumor.Proceedings of the National Academy of Sciences of the United States of America · 2026Article
- Defect Engineering Activates Pyrene-Based Covalent Organic Frameworks for Efficient Photocatalytic Uranium Capture.Advanced science (Weinheim, Baden-Wurttemberg, Germany) · 2026Article
- Scalable and straightforward synthesis of electrocatalysts for green hydrogen economy via high-current-density alkaline water splitting.National science review · 2025Review
- Defect-Engineered Multi-Intermetallic Heterostructures as Multisite Electrocatalysts for Efficient Water Splitting.Advanced science (Weinheim, Baden-Wurttemberg, Germany) · 2025Article
- High-Density Atomic Level Defect Engineering of 2D Fe-Based Metal-Organic Frameworks Boosts Oxygen and Hydrogen Evolution Reactions.Advanced science (Weinheim, Baden-Wurttemberg, Germany) · 2024Article
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Authors and funding
12 authors.
Funding
Abstract
Electrocatalysts based on metal-organic frameworks (MOFs) attracted significant attention for water splitting, while the transition between MOFs and metal oxyhydroxide poses a great challenge in identifying authentic active sites and long-term stability. Herein, we employ on-purpose defect engineering to create high-density atomic level defects on two-dimensional Fe-MOFs. The coordination number of Fe changes from 6 to 4.46, and over 28% of unsaturated Fe sites are formed in the optimized Fe-MOF. In situ characterizations of the most optimized Fe-MOF
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