ArticleFrontiers in chemistry2024
Design and synthesis of thiahelicenes for molecular electronics.
Article in Frontiers in chemistry, 2024. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 1 paper.
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3 authors.
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Abstract
The conductance of a tunneling electron through a π-conjugated molecule may be affected by the presence of different pathways in the orbital structure of the molecule, resulting in the constructive or destructive interference of the molecular wave function. This quantum interference (QI) directly translates into enhancement or suppression of conductance and offers the possibility of controlling this phenomenon through tailored synthesis. Hence, we set up synthetic methodologies to access a series of thiophene-fused helicenes with a well-defined positioning of the sulfur atoms, which control the occurrence of conducting, linearly conjugated as well as disrupted, cross-conjugated pathways. We describe these synthetic strategies and relate the expected electronic transport through our molecules to three key variables: a) the
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