ArticleNature chemistry2024
Few-femtosecond electron transfer dynamics in photoionized donor-π-acceptor molecules.
Article in Nature chemistry, 2024. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 9 papers.
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Who cites it
9 citing papers in PubMed.
- Advances in the projected forces and momenta decoherence method for attosecond nonadiabatic molecular dynamics.Faraday discussions · 2026Article
- Excitonic Engineering in 2D-SiC through Organic Donor-Acceptor Adsorption.Precision chemistry · 2026Article
- Attosecond Momentum-Resolved Resonant Inelastic X-ray Scattering for Imaging Coupled Electron-Hole Dynamics.The journal of physical chemistry letters · 2026Article
- Adsorption of organic donor-acceptor molecules on graphene/SiC preserves light-induced charge transfer.Communications chemistry · 2026Article
- Accounting for Electronic Coherences Induced by Broadband Pulses by Using Pulse-Independent Trajectories.Journal of chemical theory and computation · 2026Article
- Modeling the Evolution of Laser-Induced Electronic Coherences with Trajectory Surface Hopping.Journal of chemical theory and computation · 2025Article
- Ultrafast probing of isotope-induced explicit symmetry breaking in ethylene.Communications chemistry · 2025Article
- Coherent Excitation of the CH Stretching Vibrations in CJournal of computational chemistry · 2025Article
- Few-femtosecond electron transfer dynamics in photoionized donor-π-acceptor molecules.Nature chemistry · 2024Article
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Authors and funding
22 authors.
Funding
Abstract
The exposure of molecules to attosecond extreme-ultraviolet (XUV) pulses offers a unique opportunity to study the early stages of coupled electron-nuclear dynamics in which the role played by the different degrees of freedom is beyond standard chemical intuition. We investigate, both experimentally and theoretically, the first steps of charge-transfer processes initiated by prompt ionization in prototype donor-π-acceptor molecules, namely nitroanilines. Time-resolved measurement of this process is performed by combining attosecond XUV-pump/few-femtosecond infrared-probe spectroscopy with advanced many-body quantum chemistry calculations. We show that a concerted nuclear and electronic motion drives electron transfer from the donor group on a sub-10-fs timescale. This is followed by a sub-30-fs relaxation process due to the probing of the continuously spreading nuclear wave packet in the excited electronic states of the molecular cation. These findings shed light on the role played by electron-nuclear coupling in donor-π-acceptor systems in response to photoionization.
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