Evidence map›Paper›PMID 39321305›Full record

ArticleScience advances2024

Attosecond impulsive stimulated X-ray Raman scattering in liquid water.

Oliver Alexander, Felix Egun, Laura Rego, Ana Martinez Gutierrez, Douglas Garratt, Gustavo Adolfo Cárdenas, Juan J Nogueira, Jacob P Lee, Kaixiang Zhao, Ru-Pan Wang and 28 more

Abstract read
PubMed Full text at PMC Publisher
In one paragraph

Article in Science advances, 2024. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 3 papers.

0numbers the graph read from it
0cells of the map it votes in
3citing papers in PubMed
–field-weighted citation impact
1 · What the graph read from it

What it found

Each row is one number read from the abstract, on the scale the paper reported it, with its interval. Left of the dashed line favours the treatment, right favours the comparator. Under each row is the sentence it came from. New to these charts? A ten-minute tutorial.

The abstract states no effect estimate the extractor could read, or names no intervention and outcome on the map, so this paper lights no cell and moves no belief. It is still indexed, cited and linked below.

2 · The registry

The trial behind it

Trials whose registry record cites this paper, or whose number appears in the abstract. A trial that started after this paper was published is citing it as background, not reporting it.

Neither the registry nor the abstract names a trial number. If this is a trial report, that itself is worth knowing.

3 · Its place in the literature

Who cites it

3 citing papers in PubMed.

  1. Article
  2. Article
  3. Article
4 · The record

Corrections and comments

PubMed lists nothing against this paper. Absence here is not a guarantee, only a check that was made.

5 · Who and what money

Authors and funding

38 authors.

Oliver AlexanderDepartment of Physics, Imperial College London, Blackett Laboratory, SW7 2AZ London, UK.ORCID 0000-0001-8221-7382
Felix EgunDepartment of Physics, Imperial College London, Blackett Laboratory, SW7 2AZ London, UK.ORCID 0009-0008-9559-4281
Laura RegoDepartment of Physics, Imperial College London, Blackett Laboratory, SW7 2AZ London, UK.ORCID 0000-0002-7214-7402
Ana Martinez GutierrezDepartamento de Química, Universidad Autónoma de Madrid, 28049 Madrid, Spain.
Douglas GarrattSLAC National Accelerator Laboratory, Menlo Park, CA, USA.ORCID 0000-0002-8637-9984
Gustavo Adolfo CárdenasDepartamento de Química, Universidad Autónoma de Madrid, 28049 Madrid, Spain.ORCID 0000-0001-5223-3269
Juan J NogueiraDepartamento de Química, Universidad Autónoma de Madrid, 28049 Madrid, Spain.ORCID 0000-0001-7419-5670
Jacob P LeeDepartment of Physics, Imperial College London, Blackett Laboratory, SW7 2AZ London, UK.
Kaixiang ZhaoDepartment of Physics, Imperial College London, Blackett Laboratory, SW7 2AZ London, UK.ORCID 0009-0008-4673-9210
Ru-Pan WangCenter for Free-Electron Laser Science, Department of Physics, University of Hamburg, Luruper Chaussee 149, 22761 Hamburg, Germany.ORCID 0000-0003-4495-9881
David AyusoDepartment of Physics, Imperial College London, Blackett Laboratory, SW7 2AZ London, UK.ORCID 0000-0002-5394-5361
Jonathan C T BarnardDepartment of Physics, Imperial College London, Blackett Laboratory, SW7 2AZ London, UK.
Sandra BeauvarletSLAC National Accelerator Laboratory, Menlo Park, CA, USA.ORCID 0009-0004-0746-0664
Philip H BucksbaumStanford PULSE Institute, SLAC National Accelerator Laboratory, Menlo Park, CA, USA.ORCID 0000-0003-1258-5571
David CesarSLAC National Accelerator Laboratory, Menlo Park, CA, USA.ORCID 0000-0003-3669-1854
Ryan CoffeeSLAC National Accelerator Laboratory, Menlo Park, CA, USA.ORCID 0000-0002-2619-8823
Joseph DurisSLAC National Accelerator Laboratory, Menlo Park, CA, USA.ORCID 0000-0002-9930-1166
Leszek J FrasinskiDepartment of Physics, Imperial College London, Blackett Laboratory, SW7 2AZ London, UK.ORCID 0000-0001-9308-4925
Nils HuseCenter for Free-Electron Laser Science, Department of Physics, University of Hamburg, Luruper Chaussee 149, 22761 Hamburg, Germany.ORCID 0000-0002-3281-7600
Katarzyna M KowalczykDepartment of Physics, Imperial College London, Blackett Laboratory, SW7 2AZ London, UK.ORCID 0009-0002-8884-6061
Kirk A LarsenSLAC National Accelerator Laboratory, Menlo Park, CA, USA.ORCID 0000-0002-3252-260X
Mary MatthewsDepartment of Physics, Imperial College London, Blackett Laboratory, SW7 2AZ London, UK.ORCID 0000-0003-3683-1749
Shaul MukamelDepartments of Chemistry and Physics and Astronomy, University of California-Irvine, Irvine, CA 92697, USA.ORCID 0000-0002-6015-3135
Jordan T O'NealSLAC National Accelerator Laboratory, Menlo Park, CA, USA.
Thomas PenfoldChemistry-School of Natural and Environmental Sciences, Newcastle University, Newcastle upon Tyne NE1 7RU, UK.ORCID 0000-0003-4490-5672
Emily ThiersteinSLAC National Accelerator Laboratory, Menlo Park, CA, USA.
John W G TischDepartment of Physics, Imperial College London, Blackett Laboratory, SW7 2AZ London, UK.
James R TurnerDepartment of Physics, Imperial College London, Blackett Laboratory, SW7 2AZ London, UK.
Josh VogwellDepartment of Physics, Imperial College London, Blackett Laboratory, SW7 2AZ London, UK.ORCID 0000-0002-7343-0330
Taran DriverSLAC National Accelerator Laboratory, Menlo Park, CA, USA.ORCID 0000-0002-3761-6883
Nora BerrahPhysics department, University of Connecticut, Storrs, CT 06268, USA.ORCID 0000-0003-3231-1164
Ming-Fu LinSLAC National Accelerator Laboratory, Menlo Park, CA, USA.ORCID 0000-0001-8086-2484
Georgi L DakovskiSLAC National Accelerator Laboratory, Menlo Park, CA, USA.ORCID 0000-0003-1563-1190
Stefan P MoellerSLAC National Accelerator Laboratory, Menlo Park, CA, USA.ORCID 0000-0002-7783-3532
James P CryanSLAC National Accelerator Laboratory, Menlo Park, CA, USA.ORCID 0000-0002-7776-0919
Agostino MarinelliSLAC National Accelerator Laboratory, Menlo Park, CA, USA.ORCID 0000-0002-7248-4652
Antonio PicónDepartamento de Química, Universidad Autónoma de Madrid, 28049 Madrid, Spain.ORCID 0000-0002-6142-3440
Jonathan P MarangosDepartment of Physics, Imperial College London, Blackett Laboratory, SW7 2AZ London, UK.

Funding

No grant is acknowledged in the PubMed record.

6 · The paper itself

Abstract

We report the measurement of impulsive stimulated x-ray Raman scattering in neutral liquid water. An attosecond pulse drives the excitations of an electronic wavepacket in water molecules. The process comprises two steps: a transition to core-excited states near the oxygen atoms accompanied by transition to valence-excited states. Thus, the wavepacket is impulsively created at a specific atomic site within a few hundred attoseconds through a nonlinear interaction between the water and the x-ray pulse. We observe this nonlinear signature in an intensity-dependent Stokes Raman sideband at 526 eV. Our measurements are supported by our state-of-the-art calculations based on the polarization response of water dimers in bulk solvation and propagation of attosecond x-ray pulses at liquid density.

Identifiers

PMID39321305
PMCPMC12680135

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Read under generation 80e0d062 · epoch 390. Bibliography from PubMed, PubMed Central and OpenAlex; grants from NIH RePORTER; trial links from ClinicalTrials.gov; estimates, votes and beliefs from the OpenQuestion graph.