ArticleACS photonics2024
Emergent Optical Resonances in Atomically Phase-Patterned Semiconducting Monolayers of WS
Article in ACS photonics, 2024. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Not yet cited in PubMed.
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Authors and funding
8 authors.
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Abstract
Atomic-scale control of light-matter interactions represents the ultimate frontier for many applications in photonics and quantum technology. Two-dimensional semiconductors, including transition-metal dichalcogenides, are a promising platform to achieve such control due to the combination of an atomically thin geometry and convenient photophysical properties. Here, we demonstrate that a variety of durable polymorphic structures can be combined to generate additional optical resonances beyond the standard excitons. We theoretically predict and experimentally show that atomic-sized patches of the 1T phase within the 1H matrix form unique electronic bands that lead to the emergence of robust optical resonances with strong absorption, circularly polarized emission, and long radiative lifetimes. The atomic manipulation of two-dimensional semiconductors opens unexplored scenarios for light harvesting devices and exciton-based photonics.
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Registered trials
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