Evidence map›Paper›PMID 39252158›Full record

ArticleJournal of the American Chemical Society2024

Surface-Activated Mechano-Catalysis for Ambient Conversion of Plastic Waste.

Adrian H Hergesell, Renate J Baarslag, Claire L Seitzinger, Raghavendra Meena, Patrick Schara, Željko Tomović, Guanna Li, Bert M Weckhuysen, Ina Vollmer

Abstract read
In one paragraph

Article in Journal of the American Chemical Society, 2024. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 12 papers.

0numbers the graph read from it
0cells of the map it votes in
12citing papers in PubMed
–field-weighted citation impact
1 · What the graph read from it

What it found

Each row is one number read from the abstract, on the scale the paper reported it, with its interval. Left of the dashed line favours the treatment, right favours the comparator. Under each row is the sentence it came from. New to these charts? A ten-minute tutorial.

The abstract states no effect estimate the extractor could read, or names no intervention and outcome on the map, so this paper lights no cell and moves no belief. It is still indexed, cited and linked below.

2 · The registry

The trial behind it

Trials whose registry record cites this paper, or whose number appears in the abstract. A trial that started after this paper was published is citing it as background, not reporting it.

Neither the registry nor the abstract names a trial number. If this is a trial report, that itself is worth knowing.

3 · Its place in the literature

Who cites it

12 citing papers in PubMed.

  1. Article
  2. Article
  3. Article
  4. Article
  5. Article
  6. Review
  7. Article
  8. Article
  9. Article
  10. Article
  11. Article
  12. Review
4 · The record

Corrections and comments

PubMed lists nothing against this paper. Absence here is not a guarantee, only a check that was made.

5 · Who and what money

Authors and funding

9 authors.

Adrian H HergesellInorganic Chemistry and Catalysis Group, Institute for Sustainable and Circular Chemistry, Utrecht University, Utrecht 3584 CG, The Netherlands.ORCID 0000-0003-3071-930X
Renate J BaarslagInorganic Chemistry and Catalysis Group, Institute for Sustainable and Circular Chemistry, Utrecht University, Utrecht 3584 CG, The Netherlands.
Claire L SeitzingerInorganic Chemistry and Catalysis Group, Institute for Sustainable and Circular Chemistry, Utrecht University, Utrecht 3584 CG, The Netherlands.ORCID 0000-0002-4700-9964
Raghavendra MeenaBiobased Chemistry and Technology, Wageningen University, Wageningen 6708 WG, The Netherlands.ORCID 0000-0002-2019-8806
Patrick ScharaPolymer Performance Materials Group, Department of Chemical Engineering and Chemistry, Eindhoven University of Technology, Eindhoven 5600 MB, The Netherlands.
Željko TomovićPolymer Performance Materials Group, Department of Chemical Engineering and Chemistry, Eindhoven University of Technology, Eindhoven 5600 MB, The Netherlands.ORCID 0000-0002-7944-5728
Guanna LiBiobased Chemistry and Technology, Wageningen University, Wageningen 6708 WG, The Netherlands.ORCID 0000-0003-3031-8119
Bert M WeckhuysenInorganic Chemistry and Catalysis Group, Institute for Sustainable and Circular Chemistry, Utrecht University, Utrecht 3584 CG, The Netherlands.ORCID 0000-0001-5245-1426
Ina VollmerInorganic Chemistry and Catalysis Group, Institute for Sustainable and Circular Chemistry, Utrecht University, Utrecht 3584 CG, The Netherlands.ORCID 0000-0001-9917-1499

Funding

No grant is acknowledged in the PubMed record.

6 · The paper itself

Abstract

Improved recycling technologies can offer sustainable end-of-life options for plastic waste. While polyolefins can be converted into small hydrocarbons over acid catalysts at high temperatures, we demonstrate an alternative mechano-catalytic strategy at ambient conditions. The mechanism is fundamentally different from classical acidity-driven high-temperature approaches, exploiting mechanochemically generated radical intermediates. Surface activation of zirconia grinding spheres creates redox active surface sites directly at the point of mechanical energy input. This allows control over mechano-radical reactivity, while powder catalysts are not active. Optimized milling parameters enable the formation of 45% C

Identifiers

PMID39252158
PMCPMC11440499

What OpenQuestion holds

Textmetadata
LicenceCC BY
Read underepoch 390

Registered trials

None linked

Read under generation 80e0d062 · epoch 390. Bibliography from PubMed, PubMed Central and OpenAlex; grants from NIH RePORTER; trial links from ClinicalTrials.gov; estimates, votes and beliefs from the OpenQuestion graph.