ArticleNature communications2024
Modulation of triplet quantum coherence by guest-induced structural changes in a flexible metal-organic framework.
Article in Nature communications, 2024. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 6 papers.
What it found
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The abstract states no effect estimate the extractor could read, or names no intervention and outcome on the map, so this paper lights no cell and moves no belief. It is still indexed, cited and linked below.
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Trials whose registry record cites this paper, or whose number appears in the abstract. A trial that started after this paper was published is citing it as background, not reporting it.
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Who cites it
6 citing papers in PubMed.
- Crystalline Small Molecule-Polymer Superlattice for Spatially Isolated Tetrathiafulvalene Spin Qubit Arrays.Angewandte Chemie (International ed. in English) · 2026Article
- Enlarging Quantum Coherence of Vanadyl Spin Qubits in Zirconium Porphyrinic MOFs.Inorganic chemistry · 2026Article
- A Triple-Site GdACS applied materials & interfaces · 2025Article
- Enhancing the Optically Detected Magnetic Resonance Signal of Organic Molecular Qubits.ACS central science · 2025Article
- Phononic modulation of spin-lattice relaxation in molecular qubit frameworks.Nature communications · 2024Article
- Modulation of triplet quantum coherence by guest-induced structural changes in a flexible metal-organic framework.Nature communications · 2024Article
Corrections and comments
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Authors and funding
9 authors.
Funding
Abstract
Quantum sensing has the potential to improve the sensitivity of chemical sensing by exploiting the characteristics of qubits, which are sensitive to the external environment. Modulation of quantum coherence by target analytes can be a useful tool for quantum sensing. Using molecular qubits is expected to provide excellent sensitivity due to the proximity of the sensor to the target analyte. However, many molecular qubits are used at cryogenic temperatures, and how to make molecular qubits respond to specific analytes remains unclear. Here, we propose a material design in which the coherence time changes in response to a variety of analytes at room temperature. We used the photoexcited triplet, which can be initialized at room temperature, as qubits and introduce them to a metal-organic framework that can flexibly change its pore structure in response to guest adsorption. By changing the local molecular density around the triplet qubits by adsorption of a specific analyte, the mobility of the triplet qubit can be changed, and the coherence time can be made responsive.
Identifiers
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Registered trials
Read under generation 80e0d062 · epoch 390. Bibliography from PubMed, PubMed Central and OpenAlex; grants from NIH RePORTER; trial links from ClinicalTrials.gov; estimates, votes and beliefs from the OpenQuestion graph.