ArticleProceedings of the National Academy of Sciences of the United States of America2024
Perpendicular crossing chains enable high mobility in a noncrystalline conjugated polymer.
Article in Proceedings of the National Academy of Sciences of the United States of America, 2024. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 5 papers.
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Who cites it
5 citing papers in PubMed.
- Evidence for Photoinduced Polaron Generation in a High Persistence Length Low Bandgap Conjugated Polymer in Solution.The journal of physical chemistry. B · 2026Article
- Solvent-Tuned Aggregation and Its Limited Functional Impact in a Rigid-Rod Indacenodithiophene-Benzothiadiazole Copolymer.ACS polymers Au · 2026Article
- Models connecting microstructure and charge transport in disordered semiconducting polymers: from theories to digital design.Materials horizons · 2025Review
- Isomeric 1,4-Dihydropentalene-Containing Building Blocks for High Mobility Ladder-Type Conjugated Polymers.Angewandte Chemie (International ed. in English) · 2025Article
- Annihilation-limited long-range exciton transport in high-mobility conjugated copolymer films.Proceedings of the National Academy of Sciences of the United States of America · 2025Article
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16 authors.
Funding
Abstract
The nature of interchain π-system contacts, and their relationship to hole transport, are elucidated for the high-mobility, noncrystalline conjugated polymer C16-IDTBT by the application of scanning tunneling microscopy, molecular dynamics, and quantum chemical calculations. The microstructure is shown to favor an unusual packing motif in which paired chains cross-over one another at near-perpendicular angles. By linking to mesoscale microstructural features, revealed by coarse-grained molecular dynamics and previous studies, and performing simulations of charge transport, it is demonstrated that the high mobility of C16-IDTBT can be explained by the promotion of a highly interconnected transport network, stemming from the adoption of perpendicular contacts at the nanoscale, in combination with fast intrachain transport.
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