ArticleNational science review2024
A novel cathode interphase formation methodology by preferential adsorption of a borate-based electrolyte additive.
Article in National science review, 2024. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 7 papers.
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Who cites it
7 citing papers in PubMed.
- Tailoring the Electric Double Layer for Advanced Rechargeable Batteries: Mechanisms, Strategies, and Outlook.Angewandte Chemie (International ed. in English) · 2026Review
- A High-Humidity-Tolerant Electrolyte for High-Voltage Lithium-Metal Batteries.Small (Weinheim an der Bergstrasse, Germany) · 2026Article
- Dual-gradient metal layer for practicalizing high-energy lithium batteries.Nature communications · 2025Article
- Suspended Lithium Nitrate-Based Electrolytes: Electrostatic Interactions for Mutually Rewarding Interface Optimization Strategies.Advanced science (Weinheim, Baden-Wurttemberg, Germany) · 2025Article
- Approaching fast ion transport via anion-dipole interaction in weakly solvated electrolytes enables stable Li-plating chemistry.National science review · 2025Article
- Modulating ion-dipole interactions in nonflammable phosphonate-based electrolyte for safe and stable sodium-ion pouch cells.National science review · 2025Article
- Cosolvent electrolyte chemistries for high-voltage potassium-ion battery.National science review · 2024Article
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Authors and funding
12 authors.
Funding
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Abstract
The coupling of high-capacity cathodes and lithium metal anodes promises to be the next generation of high-energy-density batteries. However, the fast-structural degradations of the cathode and anode challenge their practical application. Herein, we synthesize an electrolyte additive, tris(2,2,3,3,3-pentafluoropropyl) borane (TPFPB), for ultra-stable lithium (Li) metal||Ni-rich layered oxide batteries. It can be preferentially adsorbed on the cathode surface to form a stable (B and F)-rich cathode electrolyte interface film, which greatly suppresses the electrolyte-cathode side reactions and improves the stability of the cathode. In addition, the electrophilicity of B atoms in TPFPB enhances the solubility of LiNO
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