ArticleEnvironmental science: atmospheres2024
Towards automated inclusion of autoxidation chemistry in models: from precursors to atmospheric implications.
Article in Environmental science: atmospheres, 2024. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 2 papers.
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The abstract states no effect estimate the extractor could read, or names no intervention and outcome on the map, so this paper lights no cell and moves no belief. It is still indexed, cited and linked below.
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Who cites it
2 citing papers in PubMed.
- Mechanism Development and Evaluation of the Gas-Phase Photooxidation of Guaiacol: Insights from a Chamber Study.ACS ES&T air · 2026Article
- A mechanistic understanding of the varying yields of highly oxygenated organic molecules.Nature communications · 2025Article
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Authors and funding
14 authors.
Funding
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Abstract
In the last few decades, atmospheric formation of secondary organic aerosols (SOA) has gained increasing attention due to their impact on air quality and climate. However, methods to predict their abundance are mainly empirical and may fail under real atmospheric conditions. In this work, a close-to-mechanistic approach allowing SOA quantification is presented, with a focus on a chain-like chemical reaction called "autoxidation". A novel framework is employed to (a) describe the gas-phase chemistry, (b) predict the products' molecular structures and (c) explore the contribution of autoxidation chemistry on SOA formation under various conditions. As a proof of concept, the method is applied to benzene, an important anthropogenic SOA precursor. Our results suggest autoxidation to explain up to 100% of the benzene-SOA formed under low-NO
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