ArticleAdvanced science (Weinheim, Baden-Wurttemberg, Germany)2024
Band Structure Engineering in 2D Metal-Organic Frameworks.
Article in Advanced science (Weinheim, Baden-Wurttemberg, Germany), 2024. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 9 papers.
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Who cites it
9 citing papers in PubMed.
- Zero-Valent Nickel Stabilized in Surface-Supported Metal-Organic Chains.Angewandte Chemie (International ed. in English) · 2026Article
- Article
- Spectroscopic Fingerprinting of Coordination-driven Spin States in Metal-organic Architectures.Chemistry (Weinheim an der Bergstrasse, Germany) · 2026Article
- Revealing the Character of Coordination Bonding in 2D Metal-Organic Frameworks.Advanced science (Weinheim, Baden-Wurttemberg, Germany) · 2025Article
- Atomically-defined on-surface synthesis of multilayer metal-organic frameworks.Communications chemistry · 2025Article
- Responsive Molecules for Organic Neuromorphic Devices: Harnessing Memory Diversification.Advanced materials (Deerfield Beach, Fla.) · 2025Review
- Substrate Stabilized Charge Transfer Scheme In Coverage Controlled 2D Metal Organic Frameworks.Small (Weinheim an der Bergstrasse, Germany) · 2025Article
- Inverse Design of 2D Altermagnetic Metal-Organic Framework Monolayers from Hückel Theory of Nonbonding Molecular Orbitals.JACS Au · 2025Article
- Band Structure Engineering in 2D Metal-Organic Frameworks.Advanced science (Weinheim, Baden-Wurttemberg, Germany) · 2024Article
Corrections and comments
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Authors and funding
12 authors.
Funding
Abstract
The design of 2D metal-organic frameworks (2D MOFs) takes advantage of the combination of the diverse electronic properties of simple organic ligands with different transition metal (TM) centers. The strong directional nature of the coordinative bonds is the basis for the structural stability and the periodic arrangement of the TM cores in these architectures. Here, direct and clear evidence that 2D MOFs exhibit intriguing energy-dispersive electronic bands with a hybrid character and distinct magnetic properties in the metal cores, resulting from the interactions between the TM electronic levels and the organic ligand π-molecular orbitals, is reported. Importantly, a method to effectively tune both the electronic structure of 2D MOFs and the magnetic properties of the metal cores by exploiting the electronic structure of distinct TMs is presented. Consequently, the ionization potential characteristic of selected TMs, particularly the relative energy position and symmetry of the 3d states, can be used to strategically engineer bands within specific metal-organic frameworks. These findings not only provide a rationale for band structure engineering in 2D MOFs but also offer promising opportunities for advanced material design.
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Registered trials
Read under generation 80e0d062 · epoch 390. Bibliography from PubMed, PubMed Central and OpenAlex; grants from NIH RePORTER; trial links from ClinicalTrials.gov; estimates, votes and beliefs from the OpenQuestion graph.