ArticleNature communications2024
Two-dimensional single-crystalline mesoporous high-entropy oxide nanoplates for efficient electrochemical biomass upgrading.
Article in Nature communications, 2024. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 7 papers.
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Who cites it
7 citing papers in PubMed.
- Two-dimensional mesoporous materials: Synthetic strategies and emerging applications.iScience · 2026Review
- Orbital Symmetry Matching in Tailored Bimetal Oxides: Steering 5-Hydroxymethylfurfural Electrooxidation via Concurrent Activation of spSmall (Weinheim an der Bergstrasse, Germany) · 2026Article
- The Remarkable Rise in High-Entropy Catalysts: A New Paradigm for Sustainable Hydrogen Production.Nanomaterials (Basel, Switzerland) · 2026Review
- High-Entropy Catalysts for Biomass-Derived Chemicals Valorization: Mechanisms, Applications, and Opportunities.Nano-micro letters · 2026Review
- Sulfur-Stabilized High Entropy Oxysulfides Enable Efficient CC Bond Cleavage in Ethylene Glycol Electrooxidation for Sustainable Plastic Upcycling to Formate.ChemSusChem · 2026Article
- Valence-tuned electron bridge enables high-yield multi-electron HMF oxidation over spinel catalysts.Nature communications · 2026Article
- Electrosynthesis of 2,5-furandicarboxylic acid from 5-hydroxymethylfurfural: mechanisms, advanced catalysts, and reaction microenvironments.Chemical science · 2026Review
Corrections and comments
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Authors and funding
5 authors.
Funding
No grant is acknowledged in the PubMed record.
Abstract
Mesoporous single crystals have received more attention than ever in catalysis-related applications due to their unique structural functions. Despite great efforts, their progress in engineering crystallinity and composition has been remarkably slower than expected. In this manuscript, a template-free strategy is developed to prepare two-dimensional high-entropy oxide (HEO) nanoplates with single-crystallinity and penetrated mesoporosity, which further ensures precise control over high-entropy compositions and crystalline phases. Single-crystalline mesoporous HEOs (SC-MHEOs) disclose high electrocatalytic performance in 5-hydroxymethylfurfural oxidation reaction (HMFOR) for efficient biomass upgrading, with remarkable HMF conversion of 99.3% and superior 2,5-furandicarboxylic acid (FDCA) selectivity of 97.7%. Moreover, with nitrate reduction as coupling cathode reaction, SC-MHEO realizes concurrent electrosynthesis of value-added FDCA and ammonia in the two-electrode cell. Our study provides a powerful paradigm for producing a library of novel mesoporous single crystals for important catalysis-related applications, especially in the two-electrode cell.
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Registered trials
Read under generation 80e0d062 · epoch 390. Bibliography from PubMed, PubMed Central and OpenAlex; grants from NIH RePORTER; trial links from ClinicalTrials.gov; estimates, votes and beliefs from the OpenQuestion graph.