Evidence map›Paper›PMID 39110786›Full record

ArticleScience advances2024

Suppressing interfacial nucleation competition through supersaturation regulation for enhanced perovskite film quality and scalability.

Gao Zhang, Bin Ding, Yong Ding, Yan Liu, Changze Yu, Lirong Zeng, Yao Wang, Xin Zhang, Meijun Liu, Qingyong Tian and 5 more

Abstract read
In one paragraph

Article in Science advances, 2024. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 5 papers.

0numbers the graph read from it
0cells of the map it votes in
5citing papers in PubMed
–field-weighted citation impact
1 · What the graph read from it

What it found

Each row is one number read from the abstract, on the scale the paper reported it, with its interval. Left of the dashed line favours the treatment, right favours the comparator. Under each row is the sentence it came from. New to these charts? A ten-minute tutorial.

The abstract states no effect estimate the extractor could read, or names no intervention and outcome on the map, so this paper lights no cell and moves no belief. It is still indexed, cited and linked below.

2 · The registry

The trial behind it

Trials whose registry record cites this paper, or whose number appears in the abstract. A trial that started after this paper was published is citing it as background, not reporting it.

Neither the registry nor the abstract names a trial number. If this is a trial report, that itself is worth knowing.

3 · Its place in the literature

Who cites it

5 citing papers in PubMed.

  1. Article
  2. Review
  3. Beyond Plasmonics: Au Nanoparticles as Electron Sinks in TiOACS applied materials & interfaces · 2026
    Article
  4. Article
  5. Article
4 · The record

Corrections and comments

PubMed lists nothing against this paper. Absence here is not a guarantee, only a check that was made.

5 · Who and what money

Authors and funding

15 authors.

Gao ZhangState Key Laboratory for Mechanical Behavior of Materials, Xi'an Jiaotong University, Xi'an, Shaanxi 710049, P.R. China.ORCID 0000-0002-4665-1824
Bin DingGroup for Molecular Engineering of Functional Materials, Institute of Chemical Sciences and Engineering, EPFL VALAIS, Sion 1950, Switzerland.ORCID 0000-0001-6798-0646
Yong DingGroup for Molecular Engineering of Functional Materials, Institute of Chemical Sciences and Engineering, EPFL VALAIS, Sion 1950, Switzerland.ORCID 0000-0002-4921-0979
Yan LiuState Key Laboratory for Mechanical Behavior of Materials, Xi'an Jiaotong University, Xi'an, Shaanxi 710049, P.R. China.ORCID 0000-0003-4373-0970
Changze YuState Key Laboratory for Mechanical Behavior of Materials, Xi'an Jiaotong University, Xi'an, Shaanxi 710049, P.R. China.
Lirong ZengState Key Laboratory for Mechanical Behavior of Materials, Xi'an Jiaotong University, Xi'an, Shaanxi 710049, P.R. China.ORCID 0009-0002-5909-5625
Yao WangState Key Laboratory for Mechanical Behavior of Materials, Xi'an Jiaotong University, Xi'an, Shaanxi 710049, P.R. China.ORCID 0009-0005-1680-4585
Xin ZhangState Key Laboratory for Mechanical Behavior of Materials, Xi'an Jiaotong University, Xi'an, Shaanxi 710049, P.R. China.ORCID 0009-0006-9763-465X
Meijun LiuState Key Laboratory for Mechanical Behavior of Materials, Xi'an Jiaotong University, Xi'an, Shaanxi 710049, P.R. China.ORCID 0000-0002-2951-7981
Qingyong TianKunshan GCL Optoelectronic Materials Co., Ltd., Kunshan, Jiangsu 215300, P.R. China.
Bin FanKunshan GCL Optoelectronic Materials Co., Ltd., Kunshan, Jiangsu 215300, P.R. China.
Qiuju LiuKunshan GCL Optoelectronic Materials Co., Ltd., Kunshan, Jiangsu 215300, P.R. China.
Guanjun YangState Key Laboratory for Mechanical Behavior of Materials, Xi'an Jiaotong University, Xi'an, Shaanxi 710049, P.R. China.ORCID 0000-0002-7753-3636
Mohammad Khaja NazeeruddinGroup for Molecular Engineering of Functional Materials, Institute of Chemical Sciences and Engineering, EPFL VALAIS, Sion 1950, Switzerland.ORCID 0000-0001-5955-4786
Bo ChenState Key Laboratory for Mechanical Behavior of Materials, Xi'an Jiaotong University, Xi'an, Shaanxi 710049, P.R. China.ORCID 0000-0002-0088-8906

Funding

No grant is acknowledged in the PubMed record.

6 · The paper itself

Abstract

The growing interest in cost-effective and high-performing perovskite solar cells (PSCs) has driven extensive research. However, the challenge lies in upscaling PSCs while maintaining high performance. This study focuses on achieving uniform and compact perovskite films without pinholes and interfacial voids during upscaling from small PSCs to large-area modules. Competition in nucleation at concavities with various angles on rough-textured substrates during the gas-pumping drying process, coupled with different drying rates across the expansive film, aggravates these issues. Consequently, substrate roughness notably influences the deposition window of compact large-area perovskite films. We propose a supersaturation regulation approach aimed at achieving compact deposition of high-quality perovskite films over large areas. This involves introducing a rapid drying strategy to induce a high-supersaturation state, thereby equalizing nucleation across diverse concavities. This breakthrough enables the production of perovskite photovoltaics with high efficiencies of 25.58, 21.86, and 20.62% with aperture areas of 0.06, 29, and 1160 square centimeters, respectively.

Identifiers

PMID39110786
PMCPMC11305371

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Read under generation 80e0d062 · epoch 390. Bibliography from PubMed, PubMed Central and OpenAlex; grants from NIH RePORTER; trial links from ClinicalTrials.gov; estimates, votes and beliefs from the OpenQuestion graph.