Evidence map›Paper›PMID 39073305›Full record

ArticleAdvanced science (Weinheim, Baden-Wurttemberg, Germany)2024

Universal Copolymerization of Crosslinked Polyether Electrolytes for All-Solid-State Lithium-Metal Batteries.

Chengjun Lei, Tiankun Zhou, Mingjie Zhang, Tingting Liu, Chen Xu, Rui Wang, Xin He, Xiao Liang

Abstract read
In one paragraph

Article in Advanced science (Weinheim, Baden-Wurttemberg, Germany), 2024. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 5 papers.

0numbers the graph read from it
0cells of the map it votes in
5citing papers in PubMed
–field-weighted citation impact
1 · What the graph read from it

What it found

Each row is one number read from the abstract, on the scale the paper reported it, with its interval. Left of the dashed line favours the treatment, right favours the comparator. Under each row is the sentence it came from. New to these charts? A ten-minute tutorial.

The abstract states no effect estimate the extractor could read, or names no intervention and outcome on the map, so this paper lights no cell and moves no belief. It is still indexed, cited and linked below.

2 · The registry

The trial behind it

Trials whose registry record cites this paper, or whose number appears in the abstract. A trial that started after this paper was published is citing it as background, not reporting it.

Neither the registry nor the abstract names a trial number. If this is a trial report, that itself is worth knowing.

3 · Its place in the literature

Who cites it

5 citing papers in PubMed.

  1. Article
  2. Review
  3. Article
  4. Article
  5. Article
4 · The record

Corrections and comments

PubMed lists nothing against this paper. Absence here is not a guarantee, only a check that was made.

5 · Who and what money

Authors and funding

8 authors.

Chengjun LeiState Key Laboratory of Chem/Bio-Sensing and Chemometrics, Joint International Research Laboratory of Energy Electrochemistry, College of Chemistry and Chemical Engineering, Hunan University, Changsha, 410082, China.ORCID https://orcid.org/0000-0001-5090-5543
Tiankun ZhouState Key Laboratory of Chem/Bio-Sensing and Chemometrics, Joint International Research Laboratory of Energy Electrochemistry, College of Chemistry and Chemical Engineering, Hunan University, Changsha, 410082, China.
Mingjie ZhangState Key Laboratory of Chem/Bio-Sensing and Chemometrics, Joint International Research Laboratory of Energy Electrochemistry, College of Chemistry and Chemical Engineering, Hunan University, Changsha, 410082, China.
Tingting LiuState Key Laboratory of Chem/Bio-Sensing and Chemometrics, Joint International Research Laboratory of Energy Electrochemistry, College of Chemistry and Chemical Engineering, Hunan University, Changsha, 410082, China.
Chen XuState Key Laboratory of Chem/Bio-Sensing and Chemometrics, Joint International Research Laboratory of Energy Electrochemistry, College of Chemistry and Chemical Engineering, Hunan University, Changsha, 410082, China.
Rui WangState Key Laboratory of Chem/Bio-Sensing and Chemometrics, Joint International Research Laboratory of Energy Electrochemistry, College of Chemistry and Chemical Engineering, Hunan University, Changsha, 410082, China.
Xin HeState Key Laboratory of Chem/Bio-Sensing and Chemometrics, Joint International Research Laboratory of Energy Electrochemistry, College of Chemistry and Chemical Engineering, Hunan University, Changsha, 410082, China.
Xiao LiangState Key Laboratory of Chem/Bio-Sensing and Chemometrics, Joint International Research Laboratory of Energy Electrochemistry, College of Chemistry and Chemical Engineering, Hunan University, Changsha, 410082, China.ORCID https://orcid.org/0000-0003-4074-340X

Funding

Major Program of the Natural Science Foundation of Hunan Province 2021JC0006National Key Research and Development Program 2022YFB3807700National Natural Science Foundation of China 22209044National Natural Science Foundation of China 51972107
6 · The paper itself

Abstract

Solid polymer electrolytes (SPEs) are pivotal in advancing the practical implementation of all-solid-state batteries. Poly(1,3-dioxane) (PDOL)-based electrolytes have attracted significant attention due to the pseudo-high conductivity achieved through sophisticated in situ polymerization methods; however, such PDOL-based electrolytes present challenges of crystallization over time and monomers residual during processing. In this study, integrating LiTFSI and LiDFOB as a universal copolymerization strategy for developing high-performance PDOL electrolytes with a wide range of epoxy crosslinkers is proposed. It is discovered that this approach leverages the protective effects of TFSI anions on the boron active center and catalyzes polymer chain growth via crosslinking. The homogenously crosslinked (benzene-centered) PDOL electrolyte exhibits remarkable thermo-mechanical stability (up to 100 °C), high ion migration number (t

Indexed as

all‐solid‐state lithium‐metal batteriescatalyzeLiTFSIPDOLuniversal copolymerization

Identifiers

PMID39073305
PMCPMC11423236

What OpenQuestion holds

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Registered trials

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Read under generation 80e0d062 · epoch 390. Bibliography from PubMed, PubMed Central and OpenAlex; grants from NIH RePORTER; trial links from ClinicalTrials.gov; estimates, votes and beliefs from the OpenQuestion graph.