Evidence map›Paper›PMID 39009571›Full record

ArticleNature communications2024

AI-NERD: Elucidation of relaxation dynamics beyond equilibrium through AI-informed X-ray photon correlation spectroscopy.

James P Horwath, Xiao-Min Lin, Hongrui He, Qingteng Zhang, Eric M Dufresne, Miaoqi Chu, Subramanian K R S Sankaranarayanan, Wei Chen, Suresh Narayanan, Mathew J Cherukara

Erratum issuedAbstract read
In one paragraph

Article in Nature communications, 2024. The graph could read no effect estimate from its abstract, so it casts no vote on the map. An erratum has been issued. Cited by 2 papers.

0numbers the graph read from it
0cells of the map it votes in
2citing papers in PubMed
–field-weighted citation impact
1 · What the graph read from it

What it found

Each row is one number read from the abstract, on the scale the paper reported it, with its interval. Left of the dashed line favours the treatment, right favours the comparator. Under each row is the sentence it came from. New to these charts? A ten-minute tutorial.

The abstract states no effect estimate the extractor could read, or names no intervention and outcome on the map, so this paper lights no cell and moves no belief. It is still indexed, cited and linked below.

2 · The registry

The trial behind it

Trials whose registry record cites this paper, or whose number appears in the abstract. A trial that started after this paper was published is citing it as background, not reporting it.

Neither the registry nor the abstract names a trial number. If this is a trial report, that itself is worth knowing.

3 · Its place in the literature

Who cites it

2 citing papers in PubMed.

  1. Review
  2. Article
4 · The record

Corrections and comments

5 · Who and what money

Authors and funding

10 authors.

James P HorwathAdvanced Photon Source, Argonne National Laboratory, Lemont, IL, USA. jhorwath@anl.gov.ORCID http://orcid.org/0000-0002-7333-3768
Xiao-Min LinCenter for Nanoscale Materials, Argonne National Laboratory, Lemont, IL, USA.ORCID http://orcid.org/0000-0002-2879-3474
Hongrui HeMaterials Science Division and Center for Molecular Engineering, Argonne National Laboratory, Lemont, IL, USA.
Qingteng ZhangAdvanced Photon Source, Argonne National Laboratory, Lemont, IL, USA.ORCID http://orcid.org/0000-0002-1600-2161
Eric M DufresneAdvanced Photon Source, Argonne National Laboratory, Lemont, IL, USA.ORCID http://orcid.org/0000-0002-2077-4754
Miaoqi ChuAdvanced Photon Source, Argonne National Laboratory, Lemont, IL, USA.ORCID http://orcid.org/0000-0002-6465-1529
Subramanian K R S SankaranarayananCenter for Nanoscale Materials, Argonne National Laboratory, Lemont, IL, USA.
Wei ChenMaterials Science Division and Center for Molecular Engineering, Argonne National Laboratory, Lemont, IL, USA.ORCID http://orcid.org/0000-0001-8906-4278
Suresh NarayananAdvanced Photon Source, Argonne National Laboratory, Lemont, IL, USA. sureshn@anl.gov.
Mathew J CherukaraAdvanced Photon Source, Argonne National Laboratory, Lemont, IL, USA. mcherukara@anl.gov.ORCID http://orcid.org/0000-0002-1475-6998

Funding

U.S. Department of Energy (DOE) DE-AC02-06CH11357
6 · The paper itself

Abstract

Understanding and interpreting dynamics of functional materials in situ is a grand challenge in physics and materials science due to the difficulty of experimentally probing materials at varied length and time scales. X-ray photon correlation spectroscopy (XPCS) is uniquely well-suited for characterizing materials dynamics over wide-ranging time scales. However, spatial and temporal heterogeneity in material behavior can make interpretation of experimental XPCS data difficult. In this work, we have developed an unsupervised deep learning (DL) framework for automated classification of relaxation dynamics from experimental data without requiring any prior physical knowledge of the system. We demonstrate how this method can be used to accelerate exploration of large datasets to identify samples of interest, and we apply this approach to directly correlate microscopic dynamics with macroscopic properties of a model system. Importantly, this DL framework is material and process agnostic, marking a concrete step towards autonomous materials discovery.

Identifiers

PMID39009571
PMCPMC11251071

What OpenQuestion holds

Textmetadata
LicenceCC BY
Read underepoch 390

Registered trials

None linked

Read under generation 80e0d062 · epoch 390. Bibliography from PubMed, PubMed Central and OpenAlex; grants from NIH RePORTER; trial links from ClinicalTrials.gov; estimates, votes and beliefs from the OpenQuestion graph.