ArticleThe journal of physical chemistry letters2024
Molecular Strong Coupling and Cavity Finesse.
Article in The journal of physical chemistry letters, 2024. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 3 papers.
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Who cites it
3 citing papers in PubMed.
- Strong light-matter interactions in hybrid polaritonic systems.Chemical communications (Cambridge, England) · 2026Review
- Enhanced Transport in Organic Semiconductors Mediated Through Interfacial Charge Transfer and Cooperative Strong Coupling.Nanophotonics (Berlin, Germany) · 2026Article
- Multiple interacting photonic modes in strongly coupled organic microcavities.Philosophical transactions. Series A, Mathematical, physical, and engineering sciences · 2024Article
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Authors and funding
6 authors.
Funding
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Abstract
Molecular strong coupling offers exciting prospects in physics, chemistry, and materials science. While attention has been focused on developing realistic models for the molecular systems, the important role played by the entire photonic mode structure of the optical cavities has been less explored. We show that the effectiveness of molecular strong coupling may be critically dependent on cavity finesse. Specifically we only see emission associated with a dispersive lower polariton for cavities with sufficient finesse. By developing an analytical model of cavity photoluminescence in a multimode structure we clarify the role of finite-finesse in polariton formation and show that lowering the finesse reduces the extent of the mixing of light and matter in polariton states. We suggest that the detailed nature of the photonic modes supported by a cavity will be as important in developing a coherent framework for molecular strong coupling as the inclusion of realistic molecular models.
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Registered trials
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