ArticleLight, science & applications2024
Entangled photons enabled ultrafast stimulated Raman spectroscopy for molecular dynamics.
Article in Light, science & applications, 2024. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 10 papers.
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Who cites it
10 citing papers in PubMed.
- Raman Spectroscopy in Cancer Diagnostics and Surgery: 25 Years of Progress from Surface-Enhanced Raman Spectroscopy to Artificial Intelligence─A Bibliometric and Visualized Study.Analytical chemistry · 2026Review
- Two-dimensional fluorescence spectroscopy with entangled photons and time- and frequency-resolved two-photon coincidence detection.Science advances · 2026Article
- From Microscopy to Nanoscopy: Contemporary Physical Methods in Mitochondrial Structural Biology.International journal of molecular sciences · 2026Review
- Correlated-photon time- and frequency-resolved optical spectroscopy.Nature communications · 2025Article
- Parts-per-quadrillion level gas molecule detection: CO-LITES sensing.Light, science & applications · 2025Article
- A high sensitive methane QEPAS sensor based on self-designed trapezoidal-head quartz tuning fork and high power diode laser.Photoacoustics · 2025Article
- Multivariate-coupled-enhanced photoacoustic spectroscopy with Chebyshev rational fractional-order filtering algorithm for trace CHPhotoacoustics · 2025Article
- The Quantum Information Science Challenge for Chemistry.The journal of physical chemistry letters · 2025Review
- Highly Sensitive T-Shaped Quartz Tuning Fork Based CHSensors (Basel, Switzerland) · 2024Article
- Raman Spectroscopy of Conical Intersections Using Entangled Photons.The journal of physical chemistry letters · 2024Article
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Authors and funding
3 authors.
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Abstract
Quantum entanglement has emerged as a great resource for studying the interactions between molecules and radiation. We propose a new scheme of stimulated Raman scattering with entangled photons. A quantum ultrafast Raman spectroscopy is developed for condensed-phase molecules, to monitor the exciton populations and coherences. Analytic results are obtained, showing an entanglement-enabled time-frequency scale not attainable by classical light. The Raman signal presents an unprecedented selectivity of molecular correlation functions, as a result of the Hong-Ou-Mandel interference. Our work suggests a new paradigm of using an unconventional interferometer as part of spectroscopy, with the potential to unveil advanced information about complex materials.
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