ArticleProceedings of the National Academy of Sciences of the United States of America2024
Organic nanoparticles with tunable size and rigidity by hyperbranching and cross-linking using microemulsion ATRP.
Article in Proceedings of the National Academy of Sciences of the United States of America, 2024. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 4 papers.
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Who cites it
4 citing papers in PubMed.
- Polymer-Grafted Nanoparticles as All-in-One Nanoplatforms.ACS polymers Au · 2026Review
- Heterogeneous photocatalyst enables large-scale broadband light-driven atom transfer radical polymerization with high oxygen and inhibitor tolerance.Nature communications · 2026Article
- Neutron Reflectometry Reveals Diffusion in Contrast-Matched Brush Particle Bilayers.ACS macro letters · 2026Article
- Oxygen-Tolerant Inverse Microemulsion and Miniemulsion PhotoATRP.ACS macro letters · 2026Article
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Authors and funding
12 authors.
Funding
Abstract
Unlike inorganic nanoparticles, organic nanoparticles (oNPs) offer the advantage of "interior tailorability," thereby enabling the controlled variation of physicochemical characteristics and functionalities, for example, by incorporation of diverse functional small molecules. In this study, a unique inimer-based microemulsion approach is presented to realize oNPs with enhanced control of chemical and mechanical properties by deliberate variation of the degree of hyperbranching or cross-linking. The use of anionic cosurfactants led to oNPs with superior uniformity. Benefitting from the high initiator concentration from inimer and preserved chain-end functionality during atom transfer radical polymerization (ATRP), the capability of oNPs as a multifunctional macroinitiator for the subsequent surface-initiated ATRP was demonstrated. This facilitated the synthesis of densely tethered poly(methyl methacrylate) brush oNPs. Detailed analysis revealed that exceptionally high grafting densities (~1 nm
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