Evidence map›Paper›PMID 38916586›Full record

ArticleJournal of the American Chemical Society2024

Mining the Carbon Intermediates in Plastic Waste Upcycling for Constructing C-S Bond.

Hongxing Kang, Dong He, Christopher Turchiano, Xingxu Yan, Jingtong Chai, Melanie Weed, Gregory I Elliott, David Onofrei, Xiaoqing Pan, Xiangheng Xiao and 1 more

Abstract read
In one paragraph

Article in Journal of the American Chemical Society, 2024. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 8 papers.

0numbers the graph read from it
0cells of the map it votes in
8citing papers in PubMed
–field-weighted citation impact
1 · What the graph read from it

What it found

Each row is one number read from the abstract, on the scale the paper reported it, with its interval. Left of the dashed line favours the treatment, right favours the comparator. Under each row is the sentence it came from. New to these charts? A ten-minute tutorial.

The abstract states no effect estimate the extractor could read, or names no intervention and outcome on the map, so this paper lights no cell and moves no belief. It is still indexed, cited and linked below.

2 · The registry

The trial behind it

Trials whose registry record cites this paper, or whose number appears in the abstract. A trial that started after this paper was published is citing it as background, not reporting it.

Neither the registry nor the abstract names a trial number. If this is a trial report, that itself is worth knowing.

3 · Its place in the literature

Who cites it

8 citing papers in PubMed.

  1. Article
  2. Article
  3. Article
  4. Review
  5. Article
  6. Article
  7. Article
  8. Article
4 · The record

Corrections and comments

PubMed lists nothing against this paper. Absence here is not a guarantee, only a check that was made.

5 · Who and what money

Authors and funding

11 authors.

Hongxing KangDepartment of Chemistry and Biochemistry, San Diego State University, 5500 Campanile Drive, San Diego, California 92182, United States.
Dong HeDepartment of Physics, Wuhan University, Wuhan, Hubei 430072, China.
Christopher TurchianoDepartment of Chemistry and Biochemistry, San Diego State University, 5500 Campanile Drive, San Diego, California 92182, United States.ORCID 0000-0003-3173-3795
Xingxu YanDepartment of Materials Science and Engineering, University of California, Irvine, California 92697, United States.ORCID 0000-0001-7991-4849
Jingtong ChaiDepartment of Chemistry and Biochemistry, San Diego State University, 5500 Campanile Drive, San Diego, California 92182, United States.
Melanie WeedDepartment of Chemistry and Biochemistry, San Diego State University, 5500 Campanile Drive, San Diego, California 92182, United States.
Gregory I ElliottDepartment of Chemistry and Biochemistry, San Diego State University, 5500 Campanile Drive, San Diego, California 92182, United States.
David OnofreiDepartment of Chemistry and Biochemistry, San Diego State University, 5500 Campanile Drive, San Diego, California 92182, United States.
Xiaoqing PanDepartment of Materials Science and Engineering, University of California, Irvine, California 92697, United States.
Xiangheng XiaoDepartment of Physics, Wuhan University, Wuhan, Hubei 430072, China.ORCID 0000-0001-9111-1619
Jing GuDepartment of Chemistry and Biochemistry, San Diego State University, 5500 Campanile Drive, San Diego, California 92182, United States.ORCID 0000-0002-5506-0049

Funding

No grant is acknowledged in the PubMed record.

6 · The paper itself

Abstract

Postconsumer plastics are generally perceived as valueless with only a small portion of plastic waste being closed-loop recycled into similar products while most of them are discarded in landfills. Depositing plastic waste in landfills not only harms the environment but also signifies a substantial economic loss. Alternatively, constructing value-added chemical feedstocks via mining the waste-derived intermediate species as a carbon (C) source under mild electrochemical conditions is a sustainable strategy to realize the circular economy. This proof-of-concept work provides an attractive "turning trash to treasure" strategy by integrating electrocatalytic polyethylene terephthalate (PET) plastic upcycling with a chemical C-S coupling reaction to synthesize organosulfur compounds, hydroxymethanesulfonate (HMS). HMS can be produced efficiently (Faradaic efficiency, FE of ∼70%) via deliberately capturing electrophilic intermediates generated in the PET monomer (ethylene glycol, EG) upcycling process, followed by coupling them with nucleophilic sulfur (S) species (i.e., SO

Identifiers

PMID38916586
PMCPMC11240564

What OpenQuestion holds

Textmetadata
LicenceCC BY-NC-ND
Read underepoch 390

Registered trials

None linked

Read under generation 80e0d062 · epoch 390. Bibliography from PubMed, PubMed Central and OpenAlex; grants from NIH RePORTER; trial links from ClinicalTrials.gov; estimates, votes and beliefs from the OpenQuestion graph.