ArticleThe journal of physical chemistry. C, Nanomaterials and interfaces2022
Thermodynamically Stable Colloidal Solids: Interfacial Thermodynamics from the Particle Size Distribution.
Article in The journal of physical chemistry. C, Nanomaterials and interfaces, 2022. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 2 papers.
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Who cites it
2 citing papers in PubMed.
- Supersaturation, Nucleation, and Phase Separation of Mesoscopic Systems.Journal of the American Chemical Society · 2025Article
- Observation of negative surface and interface energies of quantum dots.Proceedings of the National Academy of Sciences of the United States of America · 2024Article
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Authors and funding
2 authors.
Funding
Abstract
True thermodynamic stability of a solid colloidal dispersion is generally unexpected, so much that thorough experimental validation of proposed stable systems remains incomplete. Such dispersions are under investigated and would be of interest due to their long-term stability and insensitivity to preparation pathway. We apply classical nucleation theory (CNT) to such colloidal systems, providing a relationship which links the size-dependent interfacial free energy density of the particles to their size distribution, and use this expression in the fitting of previously reported size distributions for putatively thermodynamically stable nanoparticles. Experimental data from a gold-thiol system exhibiting inverse coarsening or "digestive ripening" can be well-described in terms of a power-law dependence of the interfacial free energy
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Registered trials
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