Evidence map›Paper›PMID 38871721›Full record

ArticleNature communications2024

Bubbles enable volumetric negative compressibility in metastable elastocapillary systems.

Davide Caprini, Francesco Battista, Paweł Zajdel, Giovanni Di Muccio, Carlo Guardiani, Benjamin Trump, Marcus Carter, Andrey A Yakovenko, Eder Amayuelas, Luis Bartolomé and 4 more

Abstract read
In one paragraph

Article in Nature communications, 2024. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 3 papers.

0numbers the graph read from it
0cells of the map it votes in
3citing papers in PubMed
–field-weighted citation impact
1 · What the graph read from it

What it found

Each row is one number read from the abstract, on the scale the paper reported it, with its interval. Left of the dashed line favours the treatment, right favours the comparator. Under each row is the sentence it came from. New to these charts? A ten-minute tutorial.

The abstract states no effect estimate the extractor could read, or names no intervention and outcome on the map, so this paper lights no cell and moves no belief. It is still indexed, cited and linked below.

2 · The registry

The trial behind it

Trials whose registry record cites this paper, or whose number appears in the abstract. A trial that started after this paper was published is citing it as background, not reporting it.

Neither the registry nor the abstract names a trial number. If this is a trial report, that itself is worth knowing.

3 · Its place in the literature

Who cites it

3 citing papers in PubMed.

  1. Review
  2. Article
  3. Partial Water Intrusion and Extrusion in Hydrophobic Nanopores for Thermomechanical Energy Dissipation.The journal of physical chemistry. C, Nanomaterials and interfaces · 2024
    Article
4 · The record

Corrections and comments

PubMed lists nothing against this paper. Absence here is not a guarantee, only a check that was made.

5 · Who and what money

Authors and funding

14 authors.

Davide Caprini *Center for Life Nano- & Neuro-Science, Istituto Italiano di Tecnologia, Viale Regina Elena 291, Rome, Italy.
Francesco Battista *Dipartimento di Ingegneria Meccanica e Aerospaziale, Sapienza Università di Roma, Via Eudossiana 18, Rome, Italy.ORCID http://orcid.org/0000-0001-5634-5663
Paweł Zajdel *A. Chełkowski Institute of Physics, University of Silesia, ul 75 Pułku Piechoty 1, Chorzów, Poland.ORCID http://orcid.org/0000-0003-1220-5866
Giovanni Di Muccio *Dipartimento di Ingegneria Meccanica e Aerospaziale, Sapienza Università di Roma, Via Eudossiana 18, Rome, Italy.ORCID http://orcid.org/0000-0003-1388-8806
Carlo GuardianiDipartimento di Ingegneria Meccanica e Aerospaziale, Sapienza Università di Roma, Via Eudossiana 18, Rome, Italy.ORCID http://orcid.org/0000-0002-8914-9260
Benjamin TrumpCenter for Neutron Research, National Institute of Standards and Technology, Gaithersburg, Maryland, USA.
Marcus CarterCenter for Neutron Research, National Institute of Standards and Technology, Gaithersburg, Maryland, USA.
Andrey A YakovenkoX-Ray Science Division, Advanced Photon Source, Argonne National Laboratory, Argonne, Illinois, USA.
Eder AmayuelasCentre for Cooperative Research on Alternative Energies (CIC energiGUNE), Basque Research and Technology Alliance (BRTA), Alava Technology Park, Albert Einstein 48, Vitoria-Gasteiz, Spain.
Luis BartoloméCentre for Cooperative Research on Alternative Energies (CIC energiGUNE), Basque Research and Technology Alliance (BRTA), Alava Technology Park, Albert Einstein 48, Vitoria-Gasteiz, Spain.ORCID http://orcid.org/0000-0001-9649-1470
Simone MeloniDipartimento di Scienze Chimiche e Farmaceutiche, Università degli Studi di Ferrara, Via Luigi Borsari 46, Ferrara, Italy. simone.meloni@unife.it.ORCID http://orcid.org/0000-0002-3925-3799
Yaroslav GrosuCentre for Cooperative Research on Alternative Energies (CIC energiGUNE), Basque Research and Technology Alliance (BRTA), Alava Technology Park, Albert Einstein 48, Vitoria-Gasteiz, Spain. ygrosu@cicenergigune.com.ORCID http://orcid.org/0000-0001-6523-1780
Carlo Massimo CasciolaDipartimento di Ingegneria Meccanica e Aerospaziale, Sapienza Università di Roma, Via Eudossiana 18, Rome, Italy. carlomassimo.casciola@uniroma1.it.ORCID http://orcid.org/0000-0001-8795-4517
Alberto GiacomelloDipartimento di Ingegneria Meccanica e Aerospaziale, Sapienza Università di Roma, Via Eudossiana 18, Rome, Italy. alberto.giacomello@uniroma1.it.ORCID http://orcid.org/0000-0003-2735-6982

Funding

DOE | LDRD | Argonne National Laboratory (ANL) DE-AC02-06CH11357
6 · The paper itself

Abstract

Although coveted in applications, few materials expand when subject to compression or contract under decompression, i.e., exhibit negative compressibility. A key step to achieve such counterintuitive behaviour is the destabilisations of (meta)stable equilibria of the constituents. Here, we propose a simple strategy to obtain negative compressibility exploiting capillary forces both to precompress the elastic material and to release such precompression by a threshold phenomenon - the reversible formation of a bubble in a hydrophobic flexible cavity. We demonstrate that the solid part of such metastable elastocapillary systems displays negative compressibility across different scales: hydrophobic microporous materials, proteins, and millimetre-sized laminae. This concept is applicable to fields such as porous materials, biomolecules, sensors and may be easily extended to create unexpected material susceptibilities.

Identifiers

PMID38871721
PMCPMC11176325

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Registered trials

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Read under generation 80e0d062 · epoch 390. Bibliography from PubMed, PubMed Central and OpenAlex; grants from NIH RePORTER; trial links from ClinicalTrials.gov; estimates, votes and beliefs from the OpenQuestion graph.