ArticleNature communications2024
Highly porous metal-organic framework liquids and glasses via a solvent-assisted linker exchange strategy of ZIF-8.
Article in Nature communications, 2024. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 14 papers.
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Who cites it
14 citing papers in PubMed.
- Flux-mediated ligand exchange restructures metal-organic framework glasses.Nature materials · 2026Article
- Alkali-ion-modified zeolitic imidazolate framework glasses.Nature chemistry · 2026Article
- Tailoring the Melting and Glass Transition Behavior of Zeolitic Imidazolate Frameworks via Ammonium Halide Salts.Small (Weinheim an der Bergstrasse, Germany) · 2026Article
- Nanoarchitectonics of nitrogen/selenium functionalized Co-ZIF-9(III) nanorod/nanosheet for nanomolar-level detection of nitrofurantoin antibiotics in environmental and biomedical samples.Nano convergence · 2026Article
- Effect of Ligand Substitution on the Formation of the Meltable Fe-ZIF.Materials (Basel, Switzerland) · 2026Article
- Engineering Proton Conductive Metal-Organic Glasses Through Secondary Network Formers.Small (Weinheim an der Bergstrasse, Germany) · 2026Article
- Unlocking large-area free-standing MOF-glasses for molecular sieving gas separation membranes.Nature communications · 2026Article
- Reticulating node-linker-modulator chemical spaces for modular design of alkoxide-based glasses and liquids.Nature communications · 2026Article
- Structural dynamics of melting and glass formation in a two-dimensional hybrid perovskite.Nature communications · 2025Article
- Continuous structure modification of metal-organic framework glasses via halide salts.Nature communications · 2025Article
- Liquid Coordination Polymers with Anhydrous Proton Conductivity.Angewandte Chemie (International ed. in English) · 2025Article
- Highly porous metal-organic framework glass design and application for gas separation membranes.Nature communications · 2025Article
- Binary Phase Diagrams of Coordination Polymers with Eutectic Behaviors.Journal of the American Chemical Society · 2025Article
- Functional metal-organic liquids.Chemical science · 2024Review
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Authors and funding
10 authors.
Funding
Abstract
By combining the porosity of crystalline metal-organic frameworks (MOFs) with the unique processability of the liquid state, melt-quenched MOF glasses offer exciting opportunities for molecular separation. However, progress in this field is limited by two factors. Firstly, only very few MOFs melt at elevated temperatures and transform into stable glasses upon cooling the corresponding MOF liquid. Secondly, the MOF glasses obtained thus far feature only very small porosities and very small pore sizes. Here, we demonstrate solvent-assisted linker exchange (SALE) as a versatile method to prepare highly porous melt-quenched MOF glasses from the canonical ZIF-8. Two additional organic linkers are incorporated into the non-meltable ZIF-8, yielding high-entropy, linker-exchanged ZIF-8 derivatives undergoing crystal-to-liquid-to-glass phase transitions by thermal treatment. The ZIF-8 glasses demonstrate specific pore volumes of about 0.2 cm
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