ArticleChemical science2024
Evolving better solvate electrolytes for lithium secondary batteries.
Article in Chemical science, 2024. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 2 papers.
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Who cites it
2 citing papers in PubMed.
- Element-Specific Donor Numbers for Anions.Journal of the American Chemical Society · 2026Article
- Solvent Co-Intercalation Reactions for Batteries and Beyond.Chemical reviews · 2025Review
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Authors and funding
12 authors.
Funding
No grant is acknowledged in the PubMed record.
Abstract
The overall performance of lithium batteries remains unmatched to this date. Decades of optimisation have resulted in long-lasting batteries with high energy density suitable for mobile applications. However, the electrolytes used at present suffer from low lithium transference numbers, which induces concentration polarisation and reduces efficiency of charging and discharging. Here we show how targeted modifications can be used to systematically evolve anion structural motifs which can yield electrolytes with high transference numbers. Using a multidisciplinary combination of theoretical and experimental approaches, we screened a large number of anions. Thus, we identified anions which reach lithium transference numbers around 0.9, surpassing conventional electrolytes. Specifically, we find that nitrile groups have a coordination tendency similar to SO
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Registered trials
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