Evidence map›Paper›PMID 38750165›Full record

ArticleNature nanotechnology2024

Atomic-force-microscopy-based time-domain two-dimensional infrared nanospectroscopy.

Qing Xie, Yu Zhang, Eli Janzen, James H Edgar, Xiaoji G Xu

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Article in Nature nanotechnology, 2024. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 6 papers.

0numbers the graph read from it
0cells of the map it votes in
6citing papers in PubMed
–field-weighted citation impact
1 · What the graph read from it

What it found

Each row is one number read from the abstract, on the scale the paper reported it, with its interval. Left of the dashed line favours the treatment, right favours the comparator. Under each row is the sentence it came from. New to these charts? A ten-minute tutorial.

The abstract states no effect estimate the extractor could read, or names no intervention and outcome on the map, so this paper lights no cell and moves no belief. It is still indexed, cited and linked below.

2 · The registry

The trial behind it

Trials whose registry record cites this paper, or whose number appears in the abstract. A trial that started after this paper was published is citing it as background, not reporting it.

Neither the registry nor the abstract names a trial number. If this is a trial report, that itself is worth knowing.

3 · Its place in the literature

Who cites it

6 citing papers in PubMed.

  1. Article
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4 · The record

Corrections and comments

PubMed lists nothing against this paper. Absence here is not a guarantee, only a check that was made.

5 · Who and what money

Authors and funding

5 authors.

Qing XieDepartment of Chemistry, Lehigh University, Bethlehem, PA, US.ORCID http://orcid.org/0000-0001-6996-4543
Yu ZhangAmes National Laboratory, Iowa State University, Ames, IA, US.ORCID http://orcid.org/0000-0001-7959-3213
Eli JanzenTim Taylor Department of Chemical Engineering, Kansas State University, Manhattan, KS, US.
James H EdgarTim Taylor Department of Chemical Engineering, Kansas State University, Manhattan, KS, US.ORCID http://orcid.org/0000-0003-0918-5964
Xiaoji G XuDepartment of Chemistry, Lehigh University, Bethlehem, PA, US. xgx214@lehigh.edu.ORCID http://orcid.org/0000-0003-0847-5871

Funding

Alfred P. Sloan Foundation Sloan Research FellowshipArnold and Mabel Beckman Foundation Beckman Young Investigator 2018Camille and Henry Dreyfus Foundation (Camille and Henry Dreyfus Foundation, Inc.) Camille Dreyfus Teacher-Scholar AwardNational Science Foundation (NSF) CHE 1847765United States Department of Defense | United States Navy | Office of Naval Research (ONR) N00014-22-1-2582
6 · The paper itself

Abstract

For decades, infrared (IR) spectroscopy has advanced on two distinct frontiers: enhancing spatial resolution and broadening spectroscopic information. Although atomic force microscopy (AFM)-based IR microscopy overcomes Abbe's diffraction limit and reaches sub-10 nm spatial resolutions, time-domain two-dimensional IR spectroscopy (2DIR) provides insights into molecular structures, mode coupling and energy transfers. Here we bridge the boundary between these two techniques and develop AFM-2DIR nanospectroscopy. Our method offers the spatial precision of AFM in combination with the rich spectroscopic information provided by 2DIR. This approach mechanically detects the sample's photothermal responses to a tip-enhanced femtosecond IR pulse sequence and extracts spatially resolved spectroscopic information via FFTs. In a proof-of-principle experiment, we elucidate the anharmonicity of a carbonyl vibrational mode. Further, leveraging the near-field photons' high momenta from the tip enhancement for phase matching, we photothermally probe hyperbolic phonon polaritons in isotope-enriched h

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Read under generation 80e0d062 · epoch 390. Bibliography from PubMed, PubMed Central and OpenAlex; grants from NIH RePORTER; trial links from ClinicalTrials.gov; estimates, votes and beliefs from the OpenQuestion graph.