Evidence map›Paper›PMID 38701215›Full record

ArticleScience advances2024

Inverted nucleation for photoinduced nonequilibrium melting.

Junha Hwang, Yungok Ihm, Daewoong Nam, Jaeyong Shin, Eunyoung Park, Sung Yun Lee, Heemin Lee, Seung-Phil Heo, Sangsoo Kim, Je Young Ahn and 5 more

Abstract read
In one paragraph

Article in Science advances, 2024. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 3 papers.

0numbers the graph read from it
0cells of the map it votes in
3citing papers in PubMed
–field-weighted citation impact
1 · What the graph read from it

What it found

Each row is one number read from the abstract, on the scale the paper reported it, with its interval. Left of the dashed line favours the treatment, right favours the comparator. Under each row is the sentence it came from. New to these charts? A ten-minute tutorial.

The abstract states no effect estimate the extractor could read, or names no intervention and outcome on the map, so this paper lights no cell and moves no belief. It is still indexed, cited and linked below.

2 · The registry

The trial behind it

Trials whose registry record cites this paper, or whose number appears in the abstract. A trial that started after this paper was published is citing it as background, not reporting it.

Neither the registry nor the abstract names a trial number. If this is a trial report, that itself is worth knowing.

3 · Its place in the literature

Who cites it

3 citing papers in PubMed.

  1. Article
  2. Article
  3. Review
4 · The record

Corrections and comments

PubMed lists nothing against this paper. Absence here is not a guarantee, only a check that was made.

5 · Who and what money

Authors and funding

15 authors.

Junha HwangDepartment of Physics, POSTECH, Pohang 37673, Korea.ORCID 0009-0005-9049-3981
Yungok IhmPhoton Science Center, POSTECH, Pohang 37673, Korea.ORCID 0000-0002-8070-0757
Daewoong NamPhoton Science Center, POSTECH, Pohang 37673, Korea.ORCID 0000-0002-4544-4663
Jaeyong ShinDepartment of Physics, POSTECH, Pohang 37673, Korea.
Eunyoung ParkDepartment of Physics, POSTECH, Pohang 37673, Korea.ORCID 0000-0003-3988-1004
Sung Yun LeeDepartment of Physics, POSTECH, Pohang 37673, Korea.ORCID 0000-0003-2087-500X
Heemin LeeDepartment of Physics, POSTECH, Pohang 37673, Korea.ORCID 0000-0002-8727-210X
Seung-Phil HeoDepartment of Physics, POSTECH, Pohang 37673, Korea.
Sangsoo KimPohang Accelerator Laboratory, Pohang 37673, Korea.ORCID 0000-0003-4005-5404
Je Young AhnDepartment of Chemistry, POSTECH, Pohang 37673, Korea.
Ji Hoon ShimPhoton Science Center, POSTECH, Pohang 37673, Korea.ORCID 0000-0001-7357-0029
Minseok KimPohang Accelerator Laboratory, Pohang 37673, Korea.ORCID 0000-0002-2504-1314
Intae EomPhoton Science Center, POSTECH, Pohang 37673, Korea.ORCID 0000-0002-3390-4052
Do Young NohDepartment of Physics and Photon Science, Gwangju Institute of Science and Technology, Gwangju 61005, Korea.ORCID 0000-0003-2844-3906
Changyong SongDepartment of Physics, POSTECH, Pohang 37673, Korea.ORCID 0000-0001-9950-9007

Funding

No grant is acknowledged in the PubMed record.

6 · The paper itself

Abstract

Ultrafast photoinduced melting provides an essential platform for studying nonequilibrium phase transitions by linking the kinetics of electron dynamics to ionic motions. Knowledge of dynamic balance in their energetics is essential to understanding how the ionic reaction is influenced by femtosecond photoexcited electrons with notable time lag depending on reaction mechanisms. Here, by directly imaging fluctuating density distributions and evaluating the ionic pressure and Gibbs free energy from two-temperature molecular dynamics that verified experimental results, we uncovered that transient ionic pressure, triggered by photoexcited electrons, controls the overall melting kinetics. In particular, ultrafast nonequilibrium melting can be described by the reverse nucleation process with voids as nucleation seeds. The strongly driven solid-to-liquid transition of metallic gold is successfully explained by void nucleation facilitated by photoexcited electron-initiated ionic pressure, establishing a solid knowledge base for understanding ultrafast nonequilibrium kinetics.

Identifiers

PMID38701215
PMCPMC11092333

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Read under generation 80e0d062 · epoch 390. Bibliography from PubMed, PubMed Central and OpenAlex; grants from NIH RePORTER; trial links from ClinicalTrials.gov; estimates, votes and beliefs from the OpenQuestion graph.