ArticleChemical science2024
Singlet fission in TIPS-anthracene thin films.
Article in Chemical science, 2024. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 6 papers.
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Who cites it
6 citing papers in PubMed.
- Artificial Intelligence-Driven Inverse Design of Singlet Fission Candidates in the Acene family.Advanced science (Weinheim, Baden-Wurttemberg, Germany) · 2026Article
- Harnessing Triplets of TIPS-Anthracene-Based Au(I) Complexes for Photoinduced Electron Transfer and Room-Temperature Phosphorescence.Inorganic chemistry · 2026Article
- An experimental perspective on symmetry breaking and the singlet fission mechanism in solid-state materials.Chemical science · 2026Review
- Generative design of singlet fission materials leveraging a fragment-oriented database.Chemical science · 2025Article
- Janus-Type Photophysics of Rotational Isomers in a Diphenylanthracene Dimer.Angewandte Chemie (International ed. in English) · 2025Article
- Automated Research Platform for Development of Triplet-Triplet Annihilation Photon Upconversion Systems.ACS central science · 2025Article
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Authors and funding
8 authors.
Funding
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Abstract
Singlet fission is an exciton multiplication process that allows for the conversion of one singlet exciton into two triplet excitons. Organic semiconductors, such as acenes and their soluble bis(triisopropylsilylethynyl) (TIPS) substituted counterparts, have played a major role in elucidating the understanding of the underlying mechanisms of singlet fission. Despite this, one prominent member of the acene family that has received little experimental attention to date is TIPS-anthracene, even with computational studies suggesting potential high singlet fission yields in the solid state. Here, time-resolved spectroscopic and magneto-photoluminescence measurements were performed on spin-cast films of TIPS-anthracene, showing evidence for singlet fission. A singlet fission yield of 19% (out of 200%) is estimated from transient absorption spectroscopy. Kinetic modeling of the magnetic field effect on photoluminescence suggests that fast rates of triplet dissociation lead to a low magnetic photoluminescence effect and that non-radiative decay of both the S
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