ArticleNature communications2024
Spatial decoupling of bromide-mediated process boosts propylene oxide electrosynthesis.
Article in Nature communications, 2024. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 14 papers.
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Who cites it
14 citing papers in PubMed.
- Green Propylene Electrooxidation: Bridging Catalyst Design, Multi-Energy Coupling, and Reactor Engineering.Small (Weinheim an der Bergstrasse, Germany) · 2026Review
- Bromide-mediated paired electrosynthesis of hydrogen and epoxide.Nature communications · 2026Article
- Heterogeneous Indirect Redox Electrocatalysis in Electrolyte.Advanced materials (Deerfield Beach, Fla.) · 2026Review
- Direct extraction of bromine from seawater through an electrolysis-driven styrene enrichment process.Nature communications · 2026Article
- Chlorine radical-mediated electrochemical propylene epoxidation from seawater.Nature communications · 2026Article
- An Electrocatalytic/Heterogeneous Catalytic Cascade for Selective Production of Propylene Oxide via Anodic HAngewandte Chemie (International ed. in English) · 2026Article
- The utilization of ions in seawater for electrocatalysis.National science review · 2025Review
- Homogeneous silver catalyst for propylene electrooxidation to propylene glycol.Nature communications · 2025Article
- Enhancing Cascade Reaction Efficiency by Local pH Regulation for Integrated Anodic HAngewandte Chemie (International ed. in English) · 2025Article
- A supporting-electrolyte-free four-compartment electrochemical reactor for aqueous and organic phase electrosynthesis.Proceedings of the National Academy of Sciences of the United States of America · 2025Article
- Engineered NiO/TiODiscover nano · 2025Article
- Bromide-mediated membraneless electrosynthesis of ethylene carbonate from CONature communications · 2025Article
- Universal high-efficiency electrocatalytic olefin epoxidation via a surface-confined radical promotion.Nature communications · 2024Article
- Perfluoroalkyl-modified covalent organic frameworks for continuous photocatalytic hydrogen peroxide synthesis and extraction in a biphasic fluid system.Nature communications · 2024Article
Corrections and comments
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Authors and funding
10 authors.
Funding
No grant is acknowledged in the PubMed record.
Abstract
The electrochemical synthesis of propylene oxide is far from practical application due to the limited performance (including activity, stability, and selectivity). In this work, we spatially decouple the bromide-mediated process to avoid direct contact between the anode and propylene, where bromine is generated at the anode and then transferred into an independent reactor to react with propylene. This strategy effectively prevents the side reactions and eliminates the interference to stability caused by massive alkene input and vigorously stirred electrolytes. As expected, the selectivity for propylene oxide reaches above 99.9% with a remarkable Faradaic efficiency of 91% and stability of 750-h (>30 days). When the electrode area is scaled up to 25 cm
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Registered trials
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