ArticleNature communications2024
Timescale correlation of shallow trap states increases electrochemiluminescence efficiency in carbon nitrides.
Article in Nature communications, 2024. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 12 papers.
What it found
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Who cites it
12 citing papers in PubMed.
- Synergistic sensitization between Rh-MOF and Ru(bpy)Mikrochimica acta · 2026Article
- Mechanistic insights into electrochemiluminescence: fueling advances in bioanalysis and imaging.Chemical science · 2026Review
- Self-Enhanced Dual-Emissive Electrochemiluminescent Metallacages Combining Aggregation-Caused Quenching and Aggregation-Induced Emission Dyes.Small (Weinheim an der Bergstrasse, Germany) · 2026Article
- Electrochemiluminescence Illuminates Single-Atom Catalysts: Real-Time Atomic-Scale Dynamics and Operando Electronic Fingerprinting.Small methods · 2026Review
- Portable and high-throughput electrochemiluminescence detection of catechol based on self-enhanced Au-Ru@Zn MOF with exogenous/endogenous co-reactant synergy.Mikrochimica acta · 2026Article
- Breaking the catalysis-quenching dilemma in covalent organic frameworks with metal single-atom sites for enhanced electrochemiluminescence.Nature communications · 2026Article
- A quenched electrochemiluminescence immunosensor based on luminol-Au NPs/Co-Fe-MOF and CuO@UiO-66-NHMikrochimica acta · 2026Article
- Boosting Electrochemiluminescence of Carbon Nitrides via Molecular Capacitor-Mediated Spatiotemporal Electron Coordination.Advanced science (Weinheim, Baden-Wurttemberg, Germany) · 2026Article
- Surface-enhanced electrochemiluminescence combined with resonance energy transfer for sensitive detection of microcystin-LR.Mikrochimica acta · 2025Article
- Target-responsive vesicular nanoprobe for fluorescent detection of lipase.Mikrochimica acta · 2025Article
- Exploring Surface State and Exciplex Dominated Aggregation Induced Electrochemiluminescence of Graphene Quantum Dots Prepared via Electrochemical Exfoliation.Chemphyschem : a European journal of chemical physics and physical chemistry · 2025Article
- Highly electroactive thiazolium [5,4-d]thiazol-2,5-dicarboxylic acid-silver electrochemiluminescent metal-organic frameworks: synthesis, properties and application in glutathione detection.Mikrochimica acta · 2025Article
Corrections and comments
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Authors and funding
7 authors.
Funding
Abstract
Highly efficient interconversion of different types of energy plays a crucial role in both science and technology. Among them, electrochemiluminescence, an emission of light excited by electrochemical reactions, has drawn attention as a powerful tool for bioassays. Nonetheless, the large differences in timescale among diverse charge-transfer pathways from picoseconds to seconds significantly limit the electrochemiluminescence efficiency and hamper their broad applications. Here, we report a timescale coordination strategy to improve the electrochemiluminescence efficiency of carbon nitrides by engineering shallow electron trap states via Au-N bond functionalization. Quantitative electrochemiluminescence kinetics measurements and theoretic calculations jointly disclose that Au-N bonds endow shallow electron trap states, which coordinate the timescale of the fast electron transfer in the bulk emitter and the slow redox reaction of co-reagent at diffusion layers. The shallow electron trap states ultimately accelerate the rate and kinetics of emissive electron-hole recombination, setting a new cathodic electrochemiluminescence efficiency record of carbon nitrides, and empowering a visual electrochemiluminescence sensor for nitrite ion, a typical environmental contaminant, with superior detection range and limit.
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Registered trials
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