Evidence map›Paper›PMID 38637537›Full record

ArticleNature communications2024

Understanding the charge transfer effects of single atoms for boosting the performance of Na-S batteries.

Yao-Jie Lei, Xinxin Lu, Hirofumi Yoshikawa, Daiju Matsumura, Yameng Fan, Lingfei Zhao, Jiayang Li, Shijian Wang, Qinfen Gu, Hua-Kun Liu and 7 more

Open access · goldAbstract read
In one paragraph

Article in Nature communications, 2024. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 20 papers.

0numbers the graph read from it
0cells of the map it votes in
20citing papers in PubMed
17.5field-weighted citation impact, top 1% of its field
1 · What the graph read from it

What it found

Each row is one number read from the abstract, on the scale the paper reported it, with its interval. Left of the dashed line favours the treatment, right favours the comparator. Under each row is the sentence it came from. New to these charts? A ten-minute tutorial.

The abstract states no effect estimate the extractor could read, or names no intervention and outcome on the map, so this paper lights no cell and moves no belief. It is still indexed, cited and linked below.

2 · The registry

The trial behind it

Trials whose registry record cites this paper, or whose number appears in the abstract. A trial that started after this paper was published is citing it as background, not reporting it.

Neither the registry nor the abstract names a trial number. If this is a trial report, that itself is worth knowing.

3 · Its place in the literature

Who cites it

20 citing papers in PubMed, 84 citations in OpenAlex.

  1. Article
  2. Article
  3. Review
  4. Article
  5. Review
  6. Article
  7. Review
  8. Review
  9. Article
  10. Article
  11. Review
  12. Article
  13. Article
  14. Article
  15. Article
  16. Article
  17. Review
  18. Design Strategies of SNanomaterials (Basel, Switzerland) · 2025
    Review
  19. Review
  20. Review
4 · The record

Corrections and comments

PubMed lists nothing against this paper. Absence here is not a guarantee, only a check that was made.

5 · Who and what money

Authors and funding

17 authors at 7 institutions in 4 countries.

Yao-Jie Lei *Institute for Superconducting & Electronic Materials, Australian Institute of Innovative Materials, University of Wollongong, Innovation Campus, Squires Way, North Wollongong, NSW, 2500, Australia.
Xinxin Lu *Institute for Superconducting & Electronic Materials, Australian Institute of Innovative Materials, University of Wollongong, Innovation Campus, Squires Way, North Wollongong, NSW, 2500, Australia.ORCID http://orcid.org/0000-0003-2823-5250
Hirofumi YoshikawaSchool of Science and Technology, Kwansei Gakuin University, 2-1 Gakuen, Sanda, Hyogo, 669-1337, Japan.ORCID http://orcid.org/0000-0002-0088-1579
Daiju MatsumuraSchool of Science and Technology, Kwansei Gakuin University, 2-1 Gakuen, Sanda, Hyogo, 669-1337, Japan.
Yameng FanInstitute for Superconducting & Electronic Materials, Australian Institute of Innovative Materials, University of Wollongong, Innovation Campus, Squires Way, North Wollongong, NSW, 2500, Australia.
Lingfei ZhaoInstitute for Superconducting & Electronic Materials, Australian Institute of Innovative Materials, University of Wollongong, Innovation Campus, Squires Way, North Wollongong, NSW, 2500, Australia.
Jiayang LiInstitute for Superconducting & Electronic Materials, Australian Institute of Innovative Materials, University of Wollongong, Innovation Campus, Squires Way, North Wollongong, NSW, 2500, Australia.
Shijian WangCentre for Clean Energy Technology, School of Mathematical and Physical Sciences, Faculty of Science, University of Technology Sydney, Sydney, NSW, 2007, Australia.ORCID http://orcid.org/0009-0000-0519-4842
Qinfen GuAustralian Synchrotron 800 Blackburn Road, Clayton, VIC, 3168, Australia.
Hua-Kun LiuInstitute of Energy Materials Science, University of Shanghai for Science and Technology, Shanghai, 200093, China.ORCID http://orcid.org/0000-0002-0253-647X
Shi-Xue DouInstitute of Energy Materials Science, University of Shanghai for Science and Technology, Shanghai, 200093, China.ORCID http://orcid.org/0000-0003-3824-7693
Shanmukaraj DevarajCentre for Cooperative Research on Alternative Energies (CIC EnergiGUNE) Basque Research and Technology Alliance (BRTA) Alava Technology Park Albert Einstein 48, 01510, Vitoria-Gasteiz, Spain.ORCID http://orcid.org/0000-0001-8315-2699
Teofilo RojoInorganic Chemistry Department, University of the Basque Country UPV/EHU, P.O. Box. 644, 48080, Bilbao, Spain.
Wei-Hong LaiInstitute for Superconducting & Electronic Materials, Australian Institute of Innovative Materials, University of Wollongong, Innovation Campus, Squires Way, North Wollongong, NSW, 2500, Australia. weihongl@uow.edu.au.ORCID http://orcid.org/0000-0002-8685-9662
Michel ArmandCentre for Cooperative Research on Alternative Energies (CIC EnergiGUNE) Basque Research and Technology Alliance (BRTA) Alava Technology Park Albert Einstein 48, 01510, Vitoria-Gasteiz, Spain. marmand@cicenergigune.com.ORCID http://orcid.org/0000-0002-1303-9233
Yun-Xiao WangInstitute for Superconducting & Electronic Materials, Australian Institute of Innovative Materials, University of Wollongong, Innovation Campus, Squires Way, North Wollongong, NSW, 2500, Australia. yunxiaowang@usst.edu.cn.
Guoxiu WangCentre for Clean Energy Technology, School of Mathematical and Physical Sciences, Faculty of Science, University of Technology Sydney, Sydney, NSW, 2007, Australia. Guoxiu.Wang@uts.edu.au.ORCID http://orcid.org/0000-0003-4295-8578
University of Wollongong · AUUniversity of Shanghai for Science and Technology · CNUniversity of Technology Sydney · AUCIC energiGUNE · ESKwansei Gakuin University · JPAustralian Synchrotron · AUUniversity of the Basque Country · ES

Funding

No grant is acknowledged in the PubMed record.

6 · The paper itself

Abstract

The effective flow of electrons through bulk electrodes is crucial for achieving high-performance batteries, although the poor conductivity of homocyclic sulfur molecules results in high barriers against the passage of electrons through electrode structures. This phenomenon causes incomplete reactions and the formation of metastable products. To enhance the performance of the electrode, it is important to place substitutable electrification units to accelerate the cleavage of sulfur molecules and increase the selectivity of stable products during charging and discharging. Herein, we develop a single-atom-charging strategy to address the electron transport issues in bulk sulfur electrodes. The establishment of the synergistic interaction between the adsorption model and electronic transfer helps us achieve a high level of selectivity towards the desirable short-chain sodium polysulfides during the practical battery test. These finding indicates that the atomic manganese sites have an enhanced ability to capture and donate electrons. Additionally, the charge transfer process facilitates the rearrangement of sodium ions, thereby accelerating the kinetics of the sodium ions through the electrostatic force. These combined effects improve pathway selectivity and conversion to stable products during the redox process, leading to superior electrochemical performance for room temperature sodium-sulfur batteries.

Identifiers

PMID38637537
PMCPMC11026416
OpenAlexW4394931643

What OpenQuestion holds

Textmetadata
LicenceCC BY
Read underepoch 390

Registered trials

None linked

Read under generation 80e0d062 · epoch 390. Bibliography from PubMed, PubMed Central and OpenAlex; grants from NIH RePORTER; trial links from ClinicalTrials.gov; estimates, votes and beliefs from the OpenQuestion graph.