Evidence map›Paper›PMID 38626364›Full record

ArticleAdvanced science (Weinheim, Baden-Wurttemberg, Germany)2024

From Polyester Plastics to Diverse Monomers via Low-Energy Upcycling.

Lei Ji, Jiaolong Meng, Chengliang Li, Ming Wang, Xuefeng Jiang

Abstract read
In one paragraph

Article in Advanced science (Weinheim, Baden-Wurttemberg, Germany), 2024. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 10 papers.

0numbers the graph read from it
0cells of the map it votes in
10citing papers in PubMed
–field-weighted citation impact
1 · What the graph read from it

What it found

Each row is one number read from the abstract, on the scale the paper reported it, with its interval. Left of the dashed line favours the treatment, right favours the comparator. Under each row is the sentence it came from. New to these charts? A ten-minute tutorial.

The abstract states no effect estimate the extractor could read, or names no intervention and outcome on the map, so this paper lights no cell and moves no belief. It is still indexed, cited and linked below.

2 · The registry

The trial behind it

Trials whose registry record cites this paper, or whose number appears in the abstract. A trial that started after this paper was published is citing it as background, not reporting it.

Neither the registry nor the abstract names a trial number. If this is a trial report, that itself is worth knowing.

3 · Its place in the literature

Who cites it

10 citing papers in PubMed.

  1. Article
  2. Article
  3. Article
  4. Review
  5. Chemical Upcycling of Polyphenylene Sulfide at Room Temperature.Advanced science (Weinheim, Baden-Wurttemberg, Germany) · 2026
    Article
  6. Review
  7. Article
  8. Review
  9. Article
  10. From Polyester Plastics to Diverse Monomers via Low-Energy Upcycling.Advanced science (Weinheim, Baden-Wurttemberg, Germany) · 2024
    Article
4 · The record

Corrections and comments

PubMed lists nothing against this paper. Absence here is not a guarantee, only a check that was made.

5 · Who and what money

Authors and funding

5 authors.

Lei JiState Key Laboratory of Molecular & Process Engineering, School of Chemistry and Molecular Engineering, East China Normal University, North Zhongshan Road 3663, Shanghai, 200062, China.
Jiaolong MengState Key Laboratory of Molecular & Process Engineering, School of Chemistry and Molecular Engineering, East China Normal University, North Zhongshan Road 3663, Shanghai, 200062, China.
Chengliang LiState Key Laboratory of Molecular & Process Engineering, School of Chemistry and Molecular Engineering, East China Normal University, North Zhongshan Road 3663, Shanghai, 200062, China.
Ming WangState Key Laboratory of Molecular & Process Engineering, School of Chemistry and Molecular Engineering, East China Normal University, North Zhongshan Road 3663, Shanghai, 200062, China.
Xuefeng JiangState Key Laboratory of Molecular & Process Engineering, School of Chemistry and Molecular Engineering, East China Normal University, North Zhongshan Road 3663, Shanghai, 200062, China.ORCID https://orcid.org/0000-0002-1849-6572

Funding

Fundamental Research Funds for the Central UniversitiesNational Outstanding Youth Science Fund Project of National Natural Science Foundation of China 21871089National Outstanding Youth Science Fund Project of National Natural Science Foundation of China 22071057National Outstanding Youth Science Fund Project of National Natural Science Foundation of China 22125103STCSM 22JC1401000
6 · The paper itself

Abstract

Polyester plastics, constituting over 10% of the total plastic production, are widely used in packaging, fiber, single-use beverage bottles, etc. However, their current depolymerization processes face challenges such as non-broad spectrum recyclability, lack of diversified high-value-added depolymerization products, and crucially high energy consumption. Herein, an efficient strategy is developed for dismantling the compact structure of polyester plastics to achieve diverse monomer recovery. Polyester plastics undergo swelling and decrystallization with a low depolymerization energy barrier via synergistic effects of polyfluorine/hydrogen bonding, which is further demonstrated via density functional theory calculations. The swelling process is elucidated through scanning electron microscopy analysis. Obvious destruction of the crystalline region is demonstrated through X-ray crystal diffractometry curves. PET undergoes different aminolysis efficiently, yielding nine corresponding high-value-added monomers via low-energy upcycling. Furthermore, four types of polyester plastics and five types of blended polyester plastics are closed-loop recycled, affording diverse monomers with exceeding 90% yields. Kilogram-scale depolymerization of real polyethylene terephthalate (PET) waste plastics is successfully achieved with a 96% yield.

Indexed as

chemical upcyclingpolyester plasticspolyethylene terephthalatepre‐activationtrifluoroacetic acid

Identifiers

PMID38626364
PMCPMC11220695

What OpenQuestion holds

Textmetadata
LicenceCC BY
Read underepoch 390

Registered trials

None linked

Read under generation 80e0d062 · epoch 390. Bibliography from PubMed, PubMed Central and OpenAlex; grants from NIH RePORTER; trial links from ClinicalTrials.gov; estimates, votes and beliefs from the OpenQuestion graph.