Evidence map›Paper›PMID 38615087›Full record

ArticleNature communications2024

Embedding biocatalysts in a redox polymer enhances the performance of dye-sensitized photocathodes in bias-free photoelectrochemical water splitting.

Fangwen Cheng, Olha Pavliuk, Steffen Hardt, Leigh Anna Hunt, Bin Cai, Tomas Kubart, Leif Hammarström, Nicolas Plumeré, Gustav Berggren, Haining Tian

Abstract read
PubMed Full text at PMC Publisher
In one paragraph

Article in Nature communications, 2024. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 4 papers.

0numbers the graph read from it
0cells of the map it votes in
4citing papers in PubMed
–field-weighted citation impact
1 · What the graph read from it

What it found

Each row is one number read from the abstract, on the scale the paper reported it, with its interval. Left of the dashed line favours the treatment, right favours the comparator. Under each row is the sentence it came from. New to these charts? A ten-minute tutorial.

The abstract states no effect estimate the extractor could read, or names no intervention and outcome on the map, so this paper lights no cell and moves no belief. It is still indexed, cited and linked below.

2 · The registry

The trial behind it

Trials whose registry record cites this paper, or whose number appears in the abstract. A trial that started after this paper was published is citing it as background, not reporting it.

Neither the registry nor the abstract names a trial number. If this is a trial report, that itself is worth knowing.

3 · Its place in the literature

Who cites it

4 citing papers in PubMed.

  1. Review
  2. Review
  3. Review
  4. Building Localized NADP(H) Recycling Circuits to Advance Enzyme Cascadetronics.Angewandte Chemie (International ed. in English) · 2025
    Article
4 · The record

Corrections and comments

PubMed lists nothing against this paper. Absence here is not a guarantee, only a check that was made.

5 · Who and what money

Authors and funding

10 authors.

Fangwen ChengDepartment of Chemistry─Ångström laboratory, Physical Chemistry, Uppsala University, Box 521, 75120, Uppsala, Sweden.
Olha PavliukDepartment of Chemistry─Ångström laboratory, Molecular Biomimetics, Uppsala University, Box 523, 75120, Uppsala, Sweden.ORCID http://orcid.org/0000-0002-3618-8952
Steffen HardtInstitute of Energy and Climate Research, Fundamental Electrochemistry (IEK-9), Forschungszentrum Jülich GmbH, Wilhelm-Johnen-Straße, 52425, Jülich, Germany.
Leigh Anna HuntDepartment of Chemistry─Ångström laboratory, Physical Chemistry, Uppsala University, Box 521, 75120, Uppsala, Sweden.
Bin CaiDepartment of Chemistry─Ångström laboratory, Physical Chemistry, Uppsala University, Box 521, 75120, Uppsala, Sweden.
Tomas KubartDepartment of Electrical Engineering, Solid-State Electronics, Uppsala University, Box 65, 75103, Uppsala, Sweden.ORCID http://orcid.org/0000-0003-2679-2387
Leif HammarströmDepartment of Chemistry─Ångström laboratory, Physical Chemistry, Uppsala University, Box 521, 75120, Uppsala, Sweden.ORCID http://orcid.org/0000-0002-9933-9084
Nicolas PlumeréTUM Campus Straubing for Biotechnology and Sustainability, Technical University of Munich, Uferstrasse 53, 94315, Straubing, Germany. nicolas.plumere@tum.de.ORCID http://orcid.org/0000-0002-5303-7865
Gustav BerggrenDepartment of Chemistry─Ångström laboratory, Molecular Biomimetics, Uppsala University, Box 523, 75120, Uppsala, Sweden. gustav.berggren@kemi.uu.se.ORCID http://orcid.org/0000-0002-6717-6612
Haining TianDepartment of Chemistry─Ångström laboratory, Physical Chemistry, Uppsala University, Box 521, 75120, Uppsala, Sweden. haining.tian@kemi.uu.se.ORCID http://orcid.org/0000-0001-6897-2808

Funding

EC | EU Framework Programme for Research and Innovation H2020 | H2020 Priority Excellent Science | H2020 European Research Council (H2020 Excellent Science - European Research Council) 101045008Energimyndigheten (Swedish Energy Agency) 48574-1Knut och Alice Wallenbergs Stiftelse (Knut and Alice Wallenberg Foundation) 2019.0071Wenner-Gren Foundation (Wenner-Gren Foundation for Anthropological Research, Inc.) 2021.0151Wenner-Gren Foundation (Wenner-Gren Foundation for Anthropological Research, Inc.) GFU2022-0009
6 · The paper itself

Abstract

Dye-sensitized photoelectrodes consisting of photosensitizers and molecular catalysts with tunable structures and adjustable energy levels are attractive for low-cost and eco-friendly solar-assisted synthesis of energy rich products. Despite these advantages, dye-sensitized NiO photocathodes suffer from severe electron-hole recombination and facile molecule detachment, limiting photocurrent and stability in photoelectrochemical water-splitting devices. In this work, we develop an efficient and robust biohybrid dye-sensitized NiO photocathode, in which the intermolecular charge transfer is enhanced by a redox polymer. Owing to efficient assisted electron transfer from the dye to the catalyst, the biohybrid NiO photocathode showed a satisfactory photocurrent of 141±17 μA·cm

Identifiers

PMID38615087
PMCPMC11016092

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Registered trials

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Read under generation 80e0d062 · epoch 390. Bibliography from PubMed, PubMed Central and OpenAlex; grants from NIH RePORTER; trial links from ClinicalTrials.gov; estimates, votes and beliefs from the OpenQuestion graph.