Synthesis and Characterization of Phenazine-Based Redox Center for High-Performance Polymer Poly(aryl ether sulfone)-5,10-Diphenyl-dihydrophenazine.

Qilin Wang, Xuehan Wang, Yuehui Zhai, Zhibo Zheng, Huilin Shen, Yuntao Han, Zheng Chen, Zhenhua Jiang

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In one paragraph

Article in Molecules (Basel, Switzerland), 2024. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Not yet cited in PubMed.

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8 authors.

Qilin WangEngineering Research Center of Special Engineering Plastics, Ministry of Education, National and Local Joint Engineering Laboratory for Synthetic Technology of High Performance Polymer, College of Chemistry, Jilin University, Qianjin Street 2699, Changchun 130012, China.

Xuehan WangEngineering Research Center of Special Engineering Plastics, Ministry of Education, National and Local Joint Engineering Laboratory for Synthetic Technology of High Performance Polymer, College of Chemistry, Jilin University, Qianjin Street 2699, Changchun 130012, China.ORCID 0000-0001-6217-3562

Yuehui ZhaiSchool of Materials and Energy, University of Electronic Science and Technology of China, Chengdu 611731, China.

Zhibo ZhengDepartment of Chemical Engineering and Applied Chemistry, College of Chemistry, Jilin University, Qianjin Street 2699, Changchun 130012, China.

Huilin ShenEngineering Research Center of Special Engineering Plastics, Ministry of Education, National and Local Joint Engineering Laboratory for Synthetic Technology of High Performance Polymer, College of Chemistry, Jilin University, Qianjin Street 2699, Changchun 130012, China.

Yuntao HanEngineering Research Center of Special Engineering Plastics, Ministry of Education, National and Local Joint Engineering Laboratory for Synthetic Technology of High Performance Polymer, College of Chemistry, Jilin University, Qianjin Street 2699, Changchun 130012, China.ORCID 0000-0002-6540-9857

Zheng ChenEngineering Research Center of Special Engineering Plastics, Ministry of Education, National and Local Joint Engineering Laboratory for Synthetic Technology of High Performance Polymer, College of Chemistry, Jilin University, Qianjin Street 2699, Changchun 130012, China.ORCID 0000-0002-5567-522X

Zhenhua JiangEngineering Research Center of Special Engineering Plastics, Ministry of Education, National and Local Joint Engineering Laboratory for Synthetic Technology of High Performance Polymer, College of Chemistry, Jilin University, Qianjin Street 2699, Changchun 130012, China.

Funding

Jilin Province industry key core technology research project 232655GX0104106767Jilin Provincial Department of Education Science and Technology Project JJKH20231130KJthe Major Science and Technology Projects for Independent Innovation of China FAWGroup Co., Ltd. 20220301018GXthe Major Science and Technology Projects for Independent Innovation of China FAWGroup Co., Ltd. 20220301019GX

6 · The paper itself

Abstract

Phenazine-based redox-active centers are capable of averting chemical bond rearrangements by coupling during the reaction process, leading to enhanced stabilization of the material. When introduced into a high-performance polymer with excellent physicochemical properties, they can be endowed with electrochemical properties and related prospective applications while maintaining the capabilities of the materials. In this study, a facile C-N coupling method was chosen for the synthesis of serial poly(aryl ether sulfone) materials containing phenazine-based redox-active centers and to explore their electrochemical properties. As expected, the cyclic voltammetry curves of PAS-DPPZ-60, which basically overlap after thousands of cycles, indicate the stability of the electrochemical properties. As an electrochromic material, the transmittance change in PAS-DPPZ-60 exhibits only a slight attenuation after as long as 600 cycles. Meanwhile, as an organic battery cathode material, PAS-DPPZ has a theoretical specific capacity of 126 mAh g

Indexed as

electrochromismorganic battery cathodephenazinepoly(aryl ether sulfone)

Identifiers

PMID38611897

DOI10.3390/molecules29071618

PMCPMC11013081

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