ArticleAdvanced science (Weinheim, Baden-Wurttemberg, Germany)2024
Uniaxial-Oriented Perovskite Films with Controllable Orientation.
Article in Advanced science (Weinheim, Baden-Wurttemberg, Germany), 2024. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 10 papers.
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Who cites it
10 citing papers in PubMed.
- Dual-Site-Binding Ligand-Driven (100) Orientation for Efficient and Stable Perovskite Solar Cells.Advanced materials (Deerfield Beach, Fla.) · 2026Article
- GIWAXS using microbeam applied in halide perovskite films for high spectral resolution and mapping capability.Journal of synchrotron radiation · 2026Article
- Crystallization modulation for wide-bandgap perovskites with universal defect passivation toward efficient perovskite/organic tandem photovoltaics.Nature communications · 2026Article
- Recent Advances in Wide-Bandgap Perovskite Solar Cells.Advanced materials (Deerfield Beach, Fla.) · 2025Review
- Grain-Size-Dependent Stability and Crystallographic Orientation Effects in MAFA Perovskite Thin Films.The journal of physical chemistry letters · 2025Article
- Modulating phase composition and crystallization of 2D Ruddlesden-Popper perovskite filmsRSC advances · 2025Article
- Oriented wide-bandgap perovskites for monolithic silicon-based tandems with over 1000 hours operational stability.Nature communications · 2025Article
- Crystal facet engineering in perovskite photovoltaics: the rise of (111)-oriented structures.Frontiers in chemistry · 2025Review
- Application of Metal Halide Perovskite in Internet of Things.Micromachines · 2024Review
- Uniaxial-Oriented Perovskite Films with Controllable Orientation.Advanced science (Weinheim, Baden-Wurttemberg, Germany) · 2024Article
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10 authors.
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Abstract
Perovskite films with large crystal size, preferred orientation, and facile fabrication process, combining advantages of single-crystal and polycrystalline films, have gained considerable attention recently. However, there is little research on the facet properties of perovskite films. Here, (111)- and (001)-oriented perovskite films with bandgaps ranging from 1.53 to 1.77 eV, and systematically investigated their orientation-dependent properties are achieved. The (111)-oriented films show electron-dominated traps and the (001)-oriented films show hole-dominated traps, which are related to their atomic arrangement at the surface. Compared with the (001)-oriented films, the (111)-oriented films exhibit lower work function and superior water/oxygen robustness. For the wide-bandgap films, the lattice of the (001)-oriented film provides an unobstructed passage for ion migration. Comparably, the (111)-oriented films exhibit suppressed ion migration and excellent phase stability. The optimized unencapsulated solar cells based on both (001) and (111) orientations show a similar high efficiency of ≈23%. The (111)-oriented solar cell exhibits excellent stability, maintaining 95% of its initial efficiency after 1500 h maximum power point (MPP) tracking test, and 97% initial efficiency after 3000 h aging in ambient conditions. This work paves the way for the rational design, controllable synthesis, and targeted optimization of uniaxial-oriented perovskite films for various electronic applications.
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